2024
DOI: 10.1002/chem.202402721
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Structural and Electronic Factors Controlling the Efficiency and Rate of Intersystem Crossing to the Triplet State in Thiophene Polycyclic Derivatives

Cameron Griffrith,
Sarah E. Krul,
Sean J. Hoehn
et al.

Abstract: Thiophene polycyclic derivatives are widely used in organic light‐emitting diodes, photovoltaics, and medicinal chemistry applications. Understanding the electronic and structural factors controlling their intersystem crossing rates is paramount for these applications to be successful. This study investigates the photophysical, electronic structure, and excited state dynamics of 1,2‐benzodiphenylene sulfide, benzo[b]naphtho[1,2‐d]thiophene, and benzo[b]naphtho[2,3‐d]thiophene in polar aprotic and non‐polar sol… Show more

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