“…However, only a few dozens of them have been conrmed by experiments. 13,14 The most intuitive strategy for designing new 2D ferroelectric materials is to use the structure of existing 2D ferroelectric materials in the databases as a prototype and then test different combinations of chemical elements. To date, only tens of prototypes, like CuInP 2 S 6 type, 15,16 SnTe type, 17,18 a-In 2 Se 3 type, 19,20 1T ′ -MoTe 2 type, 21,22 sliding ferroelectrics and so on, are proposed theoretically and experimentally.…”