2020
DOI: 10.1002/zaac.202000133
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Studied and Forgotten. A Fresh Look at the Li–Mn–Ge System

Abstract: The crystal structure of the ternary germanide Li2MnGe has been re‐evaluated from single‐crystal X‐ray diffraction data. This compound crystallizes in a non‐centrosymmetric superstructure of the ZrCuSiAs type (space group P4bm, Pearson code tP16), with the lattice parameters a = 6.088(4) Å, c = 6.323(4) Å. First‐principle calculations for the idealized structure predict antiferromagnetic exchange in the square Mn nets and semimetallic ground state. In addition, a new ternary phase with the composition Li2–xMn4… Show more

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