2024
DOI: 10.1002/aenm.202404655
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Tailoring Molecular Space to Navigate Phase Complexity in Cs‐Based Quasi‐2D Perovskites via Gated‐Gaussian‐Driven High‐Throughput Discovery

Minsub Um,
Sheryl L. Sanchez,
Hochan Song
et al.

Abstract: Cesium‐based quasi‐2D halide perovskites (HPs) offer promising functionalities and low‐temperature manufacturability, suited to stable tandem photovoltaics. However, the chemical interplays between the molecular spacers and the inorganic building blocks during crystallization cause substantial phase complexities in the resulting matrices. To successfully optimize and implement the quasi‐2D HP functionalities, a systematic understanding of spacer chemistry, along with the seamless navigation of the inherently d… Show more

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