2024
DOI: 10.3390/e26060527
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Time-Dependent Effective Hamiltonians for Light–Matter Interactions

Aroaldo S. Santos,
Pedro H. Pereira,
Patrícia P. Abrantes
et al.

Abstract: In this paper, we present a systematic approach to building useful time-dependent effective Hamiltonians in molecular quantum electrodynamics. The method is based on considering part of the system as an open quantum system and choosing a convenient unitary transformation based on the evolution operator. We illustrate our formalism by obtaining four Hamiltonians, each suitable to a different class of applications. We show that we may treat several effects of molecular quantum electrodynamics with a direct first… Show more

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