2024
DOI: 10.1002/adma.202412083
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Tough Polyurethane Hydrogels with a Multiple Hydrogen‐Bond Interlocked Bicontinuous Phase Structure Prepared by In Situ Water‐Induced Microphase Separation

Ruyue Wang,
Ting Xu,
Yuxuan Yang
et al.

Abstract: Hydrogels with mechanical performances similar to load‐bearing tissues are in demand for in vivo applications. In this work, inspired by the self‐assembly behavior of amphiphilic polymers, polyurethane‐based tough hydrogels with a multiple hydrogen‐bond interlocked bicontinuous phase structure through in situ water‐induced microphase separation strategy are developed, in which poly(ethylene glycol)‐based polyurethane (PEG‐PU, hydrophilic) and poly(ε‐caprolactone)‐based polyurethane (PCL‐PU, hydrophobic) are bl… Show more

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