2024
DOI: 10.1021/acs.chemmater.4c02809
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Trions Stimulate Electronic Coupling in Colloidal Quantum Dot Molecules

Jordi Llusar,
Juan I. Climente

Abstract: Recent synthetic progress has enabled the controlled fusion of colloidal CdSe/CdS quantum dots in order to form dimers, manifesting electronic coupling in their optical response. While this "artificial H 2 molecule" constitutes a milestone toward the development of nanocrystal chemistry, the strength of the coupling has proven to be smaller than intended. The reason is that, when an exciton is photoinduced in the system, the hole localizes inside the CdSe cores and captures the electron, often preventing subst… Show more

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