2012
DOI: 10.1063/1.3694286
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Tuning of mid-infrared emission of ternary PbSrTe/CdTe quantum dots

Abstract: Tunable room-temperature mid-infrared photoluminescence emission from epitaxial PbSrTe quantum dots embedded in CdTe is demonstrated. By variation of the Sr content, the emission wavelength can be tuned over the whole 3 to 1.6 μm range. Comparing the emission of PbSrTe quantum dots, quantum wells and bulk material, a one order of magnitude increase in the emission efficiency is found for the quantum dots, contrary to the bulk behavior. Theoretical modelling of the transition energies shows that at higher Sr co… Show more

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Cited by 7 publications
(1 citation statement)
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“…The identical lattice constants and very different crystal structures of PbTe and CdTe (rocksalt and zincblende, respectively) result in strong segregation, and highly symmetric PbTe QD formation [266,267]. The narrow bandgap of the PbTe results in mid-IR emission in the 2-3 μm range, tunable to shorter wavelengths with the addition of Sr, or longer with the addition of Sn, to the PbTe QDs [268,269]. The symmetric, embedded and strongly segregated nanocrystalline nature of the precipitated QDs, allows room temperature mid-IR emission from LEDs using PbTe QDs as the active region [270], though the temperature dependence of the LED I-V and emission suggests that charge transport and low-resistance contacts in the less mature IV-VI material system may prove to be challenging moving forward.…”
Section: Alternative Materials Quantum Dot and Nanocrystal Emittersmentioning
confidence: 99%
“…The identical lattice constants and very different crystal structures of PbTe and CdTe (rocksalt and zincblende, respectively) result in strong segregation, and highly symmetric PbTe QD formation [266,267]. The narrow bandgap of the PbTe results in mid-IR emission in the 2-3 μm range, tunable to shorter wavelengths with the addition of Sr, or longer with the addition of Sn, to the PbTe QDs [268,269]. The symmetric, embedded and strongly segregated nanocrystalline nature of the precipitated QDs, allows room temperature mid-IR emission from LEDs using PbTe QDs as the active region [270], though the temperature dependence of the LED I-V and emission suggests that charge transport and low-resistance contacts in the less mature IV-VI material system may prove to be challenging moving forward.…”
Section: Alternative Materials Quantum Dot and Nanocrystal Emittersmentioning
confidence: 99%