2024
DOI: 10.1002/advs.202405482
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Universal Copolymerization of Crosslinked Polyether Electrolytes for All‐Solid‐State Lithium‐Metal Batteries

Chengjun Lei,
Tiankun Zhou,
Mingjie Zhang
et al.

Abstract: Solid polymer electrolytes (SPEs) are pivotal in advancing the practical implementation of all‐solid‐state batteries. Poly(1,3‐dioxane) (PDOL)‐based electrolytes have attracted significant attention due to the pseudo‐high conductivity achieved through sophisticated in situ polymerization methods; however, such PDOL‐based electrolytes present challenges of crystallization over time and monomers residual during processing. In this study, integrating LiTFSI and LiDFOB as a universal copolymerization strategy for … Show more

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