Unveiling the Structural Effects in Hybrid Copper Phosphonate Frameworks for Selective Electrocatalytic CO2 Reduction Reaction
Poojita,
Tanmay Rom,
Preetha Chandrasekharan Meenu
et al.
Abstract:Electrochemical CO 2 reduction holds tremendous promise for transforming carbon dioxide into several value-added energy feedstocks and utilizing renewable energy sources. Herein, we have developed two novel copper-based organophosphonates for selective electrocatalytic conversion of CO 2 to CH 3 OH conversion. The two-dimensional layer structure of Cu 3 [(Hhedp) 2 (C 4 H 4 N 2 )].2H 2 O (I) and the three-dimensional Cu 3 [(H 3 hedp) 2 (C 4 H 4 N 2 ) 4 (SO 4 )].2H 2 O (II) have been isolated as single crystals … Show more
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