The coronavirus disease (COVID-19) created enormous pressure across the globe due to an increasing number of COVID-19 infected cases. All the governments' primary focus is to save humanity from this pandemic problem, and they have lockdown almost the entire nation to stop the spread of infection. This lockdown resulted in a considerable impact on the global as well as a local economy that will take a long time to perform with business as usual scenario. However, improvement in the air quality of the cities across the globe has emerged as a key benefit of this lockdown. Therefore, this study aims to assess the overall impact of social and travel lockdown in five megacities of India; Delhi, Mumbai, Chennai, Kolkata, and Bangalore. The study evaluated the spatiotemporal variations in five criteria pollutants over two time periods, i.e.