The design of a high resolution photoemission electron microscope ͑PEEM͒ for the study of magnetic materials is described. PEEM is based on imaging the photoemitted ͑secondary͒ electrons from a sample irradiated by x rays. This microscope is permanently installed at the Advanced Light Source at a bending magnet that delivers linearly polarized, and left and right circularly polarized radiation in the soft x-ray range. The microscope can utilize several contrast mechanisms to study the surface and subsurface properties of materials. A wide range of contrast mechanisms can be utilized with this instrument to form topographical, elemental, chemical, magnetic circular and linear dichroism, and polarization contrast high resolution images. The electron optical properties of the microscope are described, and some first results are presented.
Nodal‐line semimetals (NLSs) represent a new type of topological semimetallic phase beyond Weyl and Dirac semimetals in the sense that they host closed loops or open curves of band degeneracies in the Brillouin zone. Parallel to the classification of type‐I and type‐II Weyl semimetals, there are two types of NLSs. The type‐I NLS phase has been proposed and realized in many compounds, whereas the exotic type‐II NLS phase that strongly violates Lorentz symmetry has remained elusive. First‐principles calculations show that Mg 3 Bi 2 is a material candidate for the type‐II NLS. The band crossing is close to the Fermi level and exhibits the type‐II nature of the nodal line in this material. Spin–orbit coupling generates only a small energy gap (≈35 meV) at the nodal points and does not negate the band dispersion of Mg 3 Bi 2 that yields the type‐II nodal line. Based on this prediction, Mg 3 Bi 2 single crystals are synthesized and the presence of the type‐II nodal lines in the material is confirmed. The angle‐resolved photoemission spectroscopy measurements agree well with the first‐principles results below the Fermi level and thus strongly suggest Mg 3 Bi 2 as an ideal material platform for studying the as‐yet unstudied properties of type‐II nodal‐line semimetals.
Proximity-induced superconductivity in a 3D topological insulator represents a new avenue for observing zero-energy Majorana fermions inside vortex cores. Relatively small gaps and low transition temperatures of conventional s-wave superconductors put the hard constraints on these experiments. Significantly larger gaps and higher transition temperatures in cuprate superconductors might be an attractive alternative to considerably relax these constraints, but it is not clear whether the proximity effect would be effective in heterostructures involving cuprates and topological insulators. Here, we present angle-resolved photoemission studies of thin Bi2Se3 films grown in-situ on optimally doped Bi2Sr2CaCu2O 8+δ substrates that show the absence of proximity-induced gaps on the surfaces of Bi2Se3 films as thin as a 1.5 quintuple layer. These results suggest that the superconducting proximity effect between a cuprate superconductor and a topological insulator is strongly suppressed, likely due to a very short coherence length along the c-axis, incompatible crystal and pairing symmetries at the interface, small size of the topological surface state's Fermi surface and adverse effects of a strong spin-orbit coupling in the topological material.
The magnetic anisotropy in antiferromagnetic 500 A thick NiO films, before and after the establishment of an exchange bias field with Co84Fe16 ferromagnetic layers, was measured using magnetic linear dichroism in soft x-ray absorption. Both <111> textured NiO and untextured NiO films show exchange-bias induced in-plane magnetic anisotropy of nearly equal magnitude and with the Ni moment axis being nearly parallel to the exchange bias field direction. These results represent the first observation of the key step in the exchange biasing process, namely, repopulation of the antiferromagnetic domains whose magnetization axis is closest to the exchange bias field direction.
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