The transfer of information between different physical forms is a central theme in communication and computation, for example between processing entities and memory. Nowhere is this more crucial than in quantum computation [1], where great effort must be taken to protect the integrity of a fragile quantum bit (qubit) [2]. However, transfer of quantum information is particularly challenging, as the process must remain coherent at all times to preserve the quantum nature of the information [3]. Here we demonstrate the coherent transfer of a superposition state in an electron spin 'processing' qubit to a nuclear spin 'memory' qubit, using a combination of microwave and radiofrequency pulses applied to 31 P donors in an isotopically pure 28 Si crystal [4,5]. The state is left in the nuclear spin on a timescale that is long compared with the electron decoherence time and then coherently transferred back to the electron spin, thus demonstrating the 31 P nuclear spin as a solid-state quantum memory. The overall store/readout fidelity is about 90%, attributed to imperfect rotations which can be improved through the use of composite pulses [6]. The coherence lifetime of the quantum memory element at 5.5 K exceeds one second.Classically, transfer of information can include a copying step, facilitating the identification and correction of errors. However, the no-cloning theorem limits the ability to faithfully copy quantum states across different degrees of freedom [7]; thus error correction becomes more challenging than for classical information and the transfer of information must take place directly. Experimental demonstrations of such transfer include moving a trapped ion qubit in and out of a decoherence-free subspace for storage purposes [8] and optical measurements of NV centres in diamond [9].Nuclear spins are known to benefit from long coherence times compared to electron spins, but are slow to manipulate and suffer from weak thermal polarisation. A powerful model for quantum computation is thus one in which electron spins are used for processing and readout while nuclear spins are used for storage. The storage element can be a single, well-defined nuclear spin, or perhaps a bath of nearby nuclear spins [10]. 31 P donors in silicon provide an ideal combination of long-lived spin-1/2 electron [11] and nuclear spins [12], with the additional advantage of integration with existing technologies [4] and the possibility of single spin detection by electrical measurement [13,14,15]. Direct measurement of the 31 P nuclear spin by NMR has only been possible at very high doping levels (e.g. near the metal insulator transition [16]). Instead, electron-nuclear double resonance (ENDOR) can be used to excite both the electron and nuclear spin associated with the donor site, and measure the nuclear spin via the electron [17]. This was recently used to measure the nuclear spin-lattice relaxation time T 1n , which was found to follow the electron relaxation time T 1e over the range 6 to 12 K with the relationship T 1n ≈ 250T 1e [5,...
We study optically driven Rabi rotations of a quantum dot exciton transition between 5 and 50 K, and for pulse areas of up to 14π. In a high driving field regime, the decay of the Rabi rotations is nonmonotonic, and the period decreases with pulse area and increases with temperature. By comparing the experiments to a weak-coupling model of the exciton-phonon interaction, we demonstrate that the observed renormalization of the Rabi frequency is induced by fluctuations in the bath of longitudinal acoustic phonons, an effect that is a phonon analogy of the Lamb shift.
In order to model realistic quantum devices it is necessary to simulate quantum systems strongly coupled to their environment. To date, most understanding of open quantum systems is restricted either to weak system–bath couplings or to special cases where specific numerical techniques become effective. Here we present a general and yet exact numerical approach that efficiently describes the time evolution of a quantum system coupled to a non-Markovian harmonic environment. Our method relies on expressing the system state and its propagator as a matrix product state and operator, respectively, and using a singular value decomposition to compress the description of the state as time evolves. We demonstrate the power and flexibility of our approach by numerically identifying the localisation transition of the Ohmic spin-boson model, and considering a model with widely separated environmental timescales arising for a pair of spins embedded in a common environment.
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