We report on time-modulated two-body weak decays observed in the orbital electron capture of hydrogenlike 140 Pr 59+ and 142 Pm 60+ ions coasting in an ion storage ring. Using non-destructive single ion, time-resolved Schottky mass spectrometry we found that the expected exponential decay is modulated in time with a modulation period of about 7 seconds for both systems. Tentatively this observation is attributed to the coherent superposition of finite mass eigenstates of the electron neutrinos from the weak decay into a two-body final state.

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The β+ and orbital electron-capture decays of stored hydrogen- and helium-like 142Pm ions have been\ud measured. So far, such measurements have been performed with only one nucleus, namely 140Pr. The\ud electron-capture decay constant of hydrogen-like 142Pm60+ ions is about 50% larger than that of heliumlike\ud 142Pm59+ ions, which is in excellent agreement with the previous measurements in 140Pr ions and\ud with new theoretical predictions

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We report on the first measurement of the beta+ and orbital electron-capture decay rates of 140Pr nuclei with the simplest electron configurations: bare nuclei, hydrogenlike, and heliumlike ions. The measured electron-capture decay constant of hydrogenlike 140Pr58+ ions is about 50% larger than that of heliumlike 140Pr57+ ions. Moreover, 140Pr ions with one bound electron decay faster than neutral 140Pr0+ atoms with 59 electrons. To explain this peculiar observation one has to take into account the conservation of the total angular momentum, since only particular spin orientations of the nucleus and of the captured electron can contribute to the allowed decay.