We report the measurement of the thermal conductivity of a suspended single-layer graphene. The room temperature values of the thermal conductivity in the range approximately (4.84+/-0.44)x10(3) to (5.30+/-0.48)x10(3) W/mK were extracted for a single-layer graphene from the dependence of the Raman G peak frequency on the excitation laser power and independently measured G peak temperature coefficient. The extremely high value of the thermal conductivity suggests that graphene can outperform carbon nanotubes in heat conduction. The superb thermal conduction property of graphene is beneficial for the proposed electronic applications and establishes graphene as an excellent material for thermal management.
Surface plasmons are collective oscillations of electrons in metals or semiconductors that enable confinement and control of electromagnetic energy at subwavelength scales. Rapid progress in plasmonics has largely relied on advances in device nano-fabrication, whereas less attention has been paid to the tunable properties of plasmonic media. One such medium--graphene--is amenable to convenient tuning of its electronic and optical properties by varying the applied voltage. Here, using infrared nano-imaging, we show that common graphene/SiO(2)/Si back-gated structures support propagating surface plasmons. The wavelength of graphene plasmons is of the order of 200 nanometres at technologically relevant infrared frequencies, and they can propagate several times this distance. We have succeeded in altering both the amplitude and the wavelength of these plasmons by varying the gate voltage. Using plasmon interferometry, we investigated losses in graphene by exploring real-space profiles of plasmon standing waves formed between the tip of our nano-probe and the edges of the samples. Plasmon dissipation quantified through this analysis is linked to the exotic electrodynamics of graphene. Standard plasmonic figures of merit of our tunable graphene devices surpass those of common metal-based structures.
The authors reported on investigation of the thermal conductivity of graphene suspended across trenches in Si/ SiO 2 wafer. The measurements were performed using a noncontact technique based on micro-Raman spectroscopy. The amount of power dissipated in graphene and corresponding temperature rise were determined from the spectral position and integrated intensity of graphene's G mode. The extremely high thermal conductivity in the range of ϳ3080-5150 W / m K and phonon mean free path of ϳ775 nm near room temperature were extracted for a set of graphene flakes. The obtained results suggest graphene's applications as thermal management material in future nanoelectronic circuits.
Graphene is the nature's thinnest elastic membrane, with exceptional mechanical and electrical properties. We report the direct observation and creation of one-dimensional (1D) and 2D periodic ripples in suspended graphene sheets, using spontaneously and thermally induced longitudinal strains on patterned substrates, with control over their orientations and wavelengths.We also provide the first measurement of graphene's thermal expansion coefficient, which is anomalously large and negative, ~ -7x10 -6 K -1 at 300K. Our work enables novel strain-based engineering of graphene devices.
Graphene, in addition to its unique electronic and optical properties, reveals unusually high thermal conductivity. The fact that the thermal conductivity of large enough graphene sheets should be higher than that of basal planes of bulk graphite was predicted theoretically by Klemens. However, the exact mechanisms behind the drastic alteration of a material's intrinsic ability to conduct heat as its dimensionality changes from two to three dimensions remain elusive. The recent availability of high-quality few-layer graphene (FLG) materials allowed us to study dimensional crossover experimentally. Here we show that the room-temperature thermal conductivity changes from approximately 2,800 to approximately 1,300 W m(-1) K(-1) as the number of atomic planes in FLG increases from 2 to 4. We explained the observed evolution from two dimensions to bulk by the cross-plane coupling of the low-energy phonons and changes in the phonon Umklapp scattering. The obtained results shed light on heat conduction in low-dimensional materials and may open up FLG applications in thermal management of nanoelectronics.
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