Mass measurements of fission and projectile fragments, produced via 238 U and 124 Xe primary beams, have been performed with the multiple-reflection time-of-flight mass spectrometer (MR-TOF-MS) of the Fragment Separator (FRS) Ion Catcher with a mass resolving power (FWHM) of up to 410 000 and an uncertainty of down to 6 × 10 −8. The nuclides were produced and separated in flight with the fragment separator FRS at 300 to 1000 MeV/u and thermalized in a cryogenic stopping cell. The data-analysis procedure was developed to determine with highest accuracy the mass values and the corresponding uncertainties for the most challenging conditions: down to a few events in a spectrum and overlapping distributions, which can be distinguished from a single peak only by a broader peak shape. With this procedure, the resolution of low-lying isomers is increased by a factor of up to 3 compared to standard data analysis. The ground-state masses of 31 short-lived nuclides of 15 different elements with half-lives of down to 17.9 ms and count rates as low as 11 events per nuclide were determined. This is the first direct mass measurement for seven nuclides. The excitation energies and the isomer-to-groundstate ratios of six isomeric states with excitation energies of as little as 280 keV were measured. For nuclides with known mass values, the average relative deviation from the literature values is (4.5 ± 5.3) × 10 −8. The measured two-neutron separation energies and their slopes near and at the N = 126 and Z = 82 shell closures indicate a strong element-dependent binding energy of the first neutron above the closed proton shell Z = 82. The experimental results deviate strongly from the theoretical predictions, especially for N = 126 and N = 127.

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The rare-earth peak in the r-process abundance pattern depends sensitively on both the astrophysical conditions and subtle changes in nuclear structure in the region. This work takes an important step elucidating the nuclear structure and reducing the uncertainties in r-process calculations via precise atomic mass measurements at the JYFLTRAP double Penning trap. 158 Nd, 160 Pm, 162 Sm, and 164−166 Gd have been measured for the first time and the precisions for 156 Nd, 158 Pm, 162,163 Eu, 163 Gd, and 164 Tb have been improved considerably. Nuclear structure has been probed via twoneutron separation energies S2n and neutron pairing energy metrics Dn. The data do not support the existence of a subshell closure at N = 100. Neutron pairing has been found to be weaker than predicted by theoretical mass models. The impact on the calculated r-process abundances has been studied. Substantial changes resulting in a smoother abundance distribution and a better agreement with the solar r-process abundances are observed.

Published version Kirsebom, O. S.; Hukkanen, M.; Kankainen, A.; Trzaska, W. H.; Strömberg, D. F.; Martínez-Pinedo, G.; Andersen, K.; Bodewits, E.; Brown, B. A.; Canete, L.; Cederkäll, J.; Enqvist, T.; Eronen, T.; Fynbo, H. O. U.; Geldhof, S.; de Groote, R., Jenkins, D. G.; Jokinen, A.; Joshi, P.; Khanam, A.; Kostensalo, J.; Kuusiniemi, P.; Langanke, K.; Moore, I.; Munch, M.; Nesterenko, D. A.; Ovejas, J. D.; Penttilä, H.; Pohjalainen, I.; Reponen, M.; Rinta-Antila, S.; Riisager, K.; de Roubin, A.; Schotanus, P.; Srivastava, P. C.; Suhonen, J.; Swartz, J. A.; Tengblad, O.; Vilen, M.; Vínals, S.; Äystö, J. Kirsebom, O. S.; Hukkanen, M.; Kankainen, A.; Trzaska, W. H.; Strömberg, D. F.; Martínez-Pinedo, G.; Andersen, K.; Bodewits, E.; Brown, B. A.; Canete, L.; Cederkäll, J.; Enqvist, T.; Eronen, T. et al. (2019). Measurement of the 2+→0+ ground-state transition in the β decay of 20F.We report the first detection of the second-forbidden, nonunique, 2 + → 0 + , ground-state transition in the β decay of 20 F. A low-energy, mass-separated 20 F + beam produced at the IGISOL facility in Jyväskylä, Finland, was implanted in a thin carbon foil and the β spectrum measured using a magnetic transporter and a plasticscintillator detector. The β-decay branching ratio inferred from the measurement is b β = [0.41 ± 0.08(stat) ± 0.07(sys)] × 10 −5 corresponding to log f t = 10.89(11), making this one of the strongest second-forbidden, nonunique β transitions ever measured. The experimental result is supported by shell-model calculations and has significant implications for the final evolution of stars that develop degenerate oxygen-neon cores. Using the new experimental data, we argue that the astrophysical electron-capture rate on 20 Ne is now known to within better than 25% at the relevant temperatures and densities.

DTAS is a segmented total absorption γ-ray spectrometer developed for the DESPEC experiment at FAIR. It is composed of up to eighteen NaI(Tl) crystals. In this work we study the performance of this detector with laboratory sources and also under real experimental conditions. We present a procedure to reconstruct offline the sum of the energy deposited in all the crystals of the spectrometer, which is complicated by the effect of NaI(Tl) light-yield non-proportionality. The use of a system to correct for time variations of the gain in individual detector modules, based on a light pulse generator, is demonstrated. We describe also an event-based method to evaluate the summing-pileup electronic distortion in segmented spectrometers. All of this allows a careful characterization of the detector with Monte Carlo simulations that is needed to calculate the response function for the analysis of total absorption γ-ray spectroscopy data. Special attention was paid to the interaction of neutrons with the spectrometer, since they are a source of contamination in studies of β-delayed neutron emitting nuclei. sponding increase in level density implies, on the one hand, the fragmentation of the β feeding into many levels populated in the decay and, on the other hand, the fragmentation of the γ intensity between many possible cascades. Total Absorption γ-Ray Spectroscopy (TAGS) has been shown to be an accurate tool to determine β-decay intensity distributions for such nuclei far from the valley of β stability. This technique avoids the so-called Pandemonium effect [2], related to the relatively poor efficiency of HPGe detectors. Instead of detecting individual γ rays as in high-resolution exper-