Shape coexistence in the light krypton isotopes was studied in two low-energy Coulomb excitation experiments using radioactive 74 Kr and 76 Kr beams from the SPIRAL facility at GANIL. The ground-state bands in both isotopes were populated up to the 8 + state via multi-step Coulomb excitation, and several non-yrast states were observed. Large sets of matrix elements were extracted for both nuclei from the observed γ -ray yields. Diagonal matrix elements were determined by utilizing the reorientation effect. In both isotopes the spectroscopic quadrupole moments for the ground-state bands and the bands based on excited 0 + 2 states are found to have opposite signs. The experimental data are interpreted within a phenomenological two-band mixing model and model-independent quadrupole invariants are deduced for the relevant 0 + states using the complete sets of matrix elements and the formalism of quadrupole sum rules. Configuration mixing calculations based on triaxial Hartree-Fock-Bogolyubov calculations with the Gogny D1S effective interaction have been performed and are compared both with the experimental results and with recent calculations using the Skyrme SLy6 effective interaction and the full generator-coordinate method restricted to axial shapes.

The Coulomb excitation experiment to study electromagnetic properties of the heaviest stable Mo isotope, 100 Mo, was performed using a 76 MeV 32 S beam from the Warsaw cyclotron U-200P. Magnitudes and relative signs of 26 E1, E2, E3, and M1 matrix elements coupling nine low-lying states in 100 Mo were determined using the least-squares code GOSIA. Diagonal matrix elements (related to the spectroscopic quadrupole moments) of the 2 + 1 , 2 + 2 , and 2 + 3 states as well as the 4 + 1 state were extracted. The resulting set of reduced E2 matrix elements was complete and precise enough to obtain, using the quadrupole sum rules approach, quadrupole deformation parameters of 100 Mo in its two lowest 0 + states: ground and excited. The overall deformation of the 0 + 1 and 0 + 2 states in 100 Mo is of similar magnitude, in both cases larger compared to what was found for the neighboring isotopes 96 Mo and 98 Mo. At the same time, the asymetry parameters obtained for both states strongly differ, indicating a triaxial shape of the 100 Mo nucleus in the ground state and a prolate shape in the excited 0 + state. Low-energy quadrupole excitations of the 100 Mo nucleus were studied in the frame of the general quadrupole collective Bohr Hamiltonian model (GBH). The potential energy and inertial functions were calculated using the adiabatic time-dependent Hartree-Fock-Bogoliubov (ATDHFB) method starting from two possible variants of the Skyrme effective interaction: SIII and Sly4. The overall quadrupole deformation parameters resulting from the GBH calculations with the SLy4 variant of the Skyrme interaction are slightly closer to the experimentally obtained values than those obtained using SIII.