We propose to install a storage ring at an ISOL-type radioactive beam facility for the first time. Specifically, we intend to install the heavy-ion, low-energy ring TSR at the HIE-ISOLDE facility in CERN, Geneva. Such a facility will provide a capability for experiments with stored secondary beams that is unique in the world. The envisaged physics programme is rich and varied, spanning from investigations of nuclear groundstate properties and reaction studies of astrophysical relevance, to investigations with highly-charged ions and pure isomeric beams. The TSR can also be used to remove isobaric contaminants from stored ion beams and for systematic studies within the neutrino beam programme. In addition to experiments performed using beams recirculating within the ring, cooled beams can also be extracted and exploited by external spectrometers for high-precision measurements. The existing TSR, which is presently in operation at the Max-Planck Institute for Nuclear Physics in Heidelberg, is well-suited and can be employed for this purpose. The physics cases, technical details of the existing ring facility and of the beam requirements at HIE-ISOLDE, together with the cost, time and manpower estimates for the transfer, installation and commissioning of the TSR at ISOLDE are discussed in the present technical design report.
The masses of very neutron-deficient nuclides close to the astrophysical rp-and νp-process paths have been determined with the Penning trap facilities JYFLTRAP at JYFL/Jyväskylä and SHIP-TRAP at GSI/Darmstadt. Isotopes from yttrium (Z = 39) to palladium (Z = 46) have been produced in heavy-ion fusion-evaporation reactions. In total 21 nuclides were studied and almost half of the mass values were experimentally determined for the first time:88 Tc,
The nuclides 104-108Sn, 106-110Sb, 108,109Te, and 111I at the expected endpoint of the astrophysical rp process have been produced in 58Ni+natNi fusion-evaporation reactions at IGISOL and their mass values were precisely measured with the JYFLTRAP Penning trap mass spectrometer. For 106Sb, 108Sb, and 110Sb these are the first direct experimental mass results obtained. The related one-proton separation energies have been derived and the value for 106Sb, Sp=424(8) keV, shows that the branching into the closed SnSbTe cycle in the astrophysical rp process is weaker than expected.
The feeding probability of 102;104;105;106;107 Tc, 105 Mo, and 101 Nb nuclei, which are important contributors to the decay heat in nuclear reactors, has been measured using the total absorption technique. We have coupled for the first time a total absorption spectrometer to a Penning trap in order to obtain sources of very high isobaric purity. Our results solve a significant part of a long-standing discrepancy in the component of the decay heat for 239 Pu in the 4-3000 s range. DOI: 10.1103/PhysRevLett.105.202501 PACS numbers: 23.40.Às, 27.60.+j, 28.41.Fr, 29.30.Kv Nuclear reactors provide a significant fraction of the world's electricity. A burgeoning population and an associated growth in economic activity suggest that world demand will double by 2050. Until now, the bulk of this has come from the burning of fossil fuels. There is general concern that reserves of fossil fuels are limited and their burning damages the environment. In particular, it contributes to the emission of large amounts of CO 2 . In this context, nuclear power, based on the fission process, will be less damaging to the environment. Accordingly there is now a renaissance in the building of nuclear power stations around the world. Modern reactor designs, based on many years of operating experience, are much more efficient, more economical, and safer than earlier designs. Although the basic principles are well established, we still lack certain information, such as a knowledge of the decay properties of specific nuclei that are important contributors to the heating of the reactor during and after operation. The estimation and control of the heat emitted by the decay of fission products plays a key role in the safe operation of reactors. The primary aim of this work is to study the decay properties of specific nuclei that are important contributors to this source of heat.Approximately 8% of the total energy generated during the fission process is related to the energy released in the natural decay of fission products, and is commonly called decay heat [1]. Once the reactor is shut down, the energy released in radioactive decay provides the main source of heating. Hence, coolant needs to be maintained after termination of the neutron-induced fission process in a reactor, and the form and extent of this essential requirement needs to be specified on the basis of decay-heat summation calculations. Decay heat varies as a function of time after shutdown and can be determined theoretically from known nuclear data. Such computations are based on the inventory of nuclei created during the fission process and after reactor shutdown and their radioactive decay characteristics:where fðtÞ is the power function, E i is the mean decay energy of the ith nuclide ( , , and components), i is the decay constant of the ith nuclide, and N i ðtÞ is the number of nuclide i at cooling time t. These calculations require extensive libraries of cross sections, fission yields, and decay data. Obviously, an accurate assessment of the decay heat is highly relevant...
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