The neutron-rich lead isotopes, up to 216 Pb, have been studied for the first time, exploiting the fragmentation of a primary uranium beam at the FRS-RISING setup at GSI. The observed isomeric states exhibit electromagnetic transition strengths which deviate from state-of-the-art shell-model calculations. It is shown that their complete description demands the introduction of effective three-body interactions and two-body transition operators in the conventional neutron valence space beyond 208 Pb. The shell model is nowadays able to provide a comprehensive view of the atomic nucleus [1]. It is a many-body theoretical framework, successful in explaining various features of the structure of nuclei, based on the definition of a restricted valence space where a suitable Hamiltonian can be diagonalized. This effective interaction originates from realistic two-body nuclear forces based on phenomenological nucleon-nucleon potentials, renormalized to be adapted to the truncated model space. Although the renormalization process can be treated in a rigorous mathematical way, the appearance of effective terms is often neglected in calculations, as a common but incorrect practice. The presence and relevance of these effective forces is well known also in other fields of physics, as for example in condensed matter studies [2]. Indeed, effective three-body terms appear already at the lower perturbation order [3]: PRL 109, 162502 (2012) P H Y S I C A L
Neutron-rich isotopes around lead, beyond N=126, have been studied exploiting the fragmentation of an uranium primary beam at the FRS-RISING setup at GSI. For the first time β-decay half-lives of 219 Bi and 211,212,213 Tl isotopes have been derived. The half-lives have been extracted using a numerical simulation developed for experiments in high-background conditions. Comparison with state of the art models used in r-process calculations is given, showing a systematic underestimation of the experimental values, at variance from close-lying nuclei.
The fragmentation of relativistic uranium projectiles has been exploited at the Gesellschaft für Schwerionenforschung laboratory to investigate the β decay of neutron-rich nuclei just beyond 208 Pb. This paper reports on β-delayed γ decays of [211][212][213] Tl, 215 Pb, and 215-219 Bi de-exciting states in the daughters 211-213 Pb, 215 Bi, and 215-219 Po. The resulting partial level schemes, proposed with the help of systematics and shell-model calculations, are presented. The role of allowed Gamow-Teller and first-forbidden β transitions in this mass region is discussed.
Neutron-rich nuclei in the lead region, beyond N = 126, have been studied at the FRS-RISING setup at GSI, exploiting the fragmentation of a primary uranium beam. Two isomeric states have been identified in 210 Hg: the 8 + isomer expected from the seniority scheme in the νg 9/2 shell and a second one at low spin and low excitation energy. The decay strength of the 8 + isomer confirms the need of effective three-body forces in the case of neutron-rich lead isotopes. The other unexpected low-lying isomer has been tentatively assigned as a 3 − state, although this is in contrast with theoretical expectations. Keywords:Atomic nuclei are complex many-body systems with many degrees of freedom; nevertheless their spectral properties often show very regular features due to the symmetries of the nuclear hamiltonian. A remarkable example of this is offered by the occurrence of the seniority excitation scheme in spherical, semi-magic nuclei [1]. A deviation from this regular behaviour suggests a change in the underlying nuclear structure,
Background: In the neutron-rich A ≈ 100 mass region, rapid shape changes as a function of nucleon number as well as coexistence of prolate, oblate, and triaxial shapes are predicted by various theoretical models. Lifetime measurements of excited levels in the molybdenum isotopes allow the determination of transitional quadrupole moments, which in turn provides structural information regarding the predicted shape change. Purpose: The present paper reports on the experimental setup, the method that allowed one to measure the lifetimes of excited states in even-even molybdenum isotopes from mass A = 100 up to mass A = 108, and the results that were obtained. Method:The isotopes of interest were populated by secondary knock-out reaction of neutron-rich nuclei separated and identified by the GSI fragment separator at relativistic beam energies and detected by the sensitive PreSPEC-AGATA experimental setup. The latter included the Lund-York-Cologne calorimeter for identification, tracking, and velocity measurement of ejectiles, and AGATA, an array of position sensitive segmented HPGe detectors, used to determine the interaction positions of the γ ray enabling a precise Doppler correction. The lifetimes were determined with a relativistic version of the Doppler-shift-attenuation method using the systematic shift of the energy after Doppler correction of a γ -ray transition with a known energy. This relativistic Doppler-shiftattenuation method allowed the determination of mean lifetimes from 2 to 250 ps. Results: Even-even molybdenum isotopes from mass A = 100 to A = 108 were studied. The decays of the low-lying states in the ground-state band were observed. In particular, two mean lifetimes were measured for the first time: τ = 29.7 Conclusions:The reduced transition strengths B(E2), calculated from lifetimes measured in this experiment, compared to beyond-mean-field calculations, indicate a gradual shape transition in the chain of molybdenum isotopes when going from A = 100 to A = 108 with a maximum reached at N = 64. The transition probabilities decrease for 108 Mo which may be related to its well-pronounced triaxial shape indicated by the calculations.
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