HAL is a multidisciplinary open access archive for the deposit and dissemination of scientific research documents, whether they are published or not. The documents may come from teaching and research institutions in France or abroad, or from public or private research centers. L'archive ouverte pluridisciplinaire HAL, est destinée au dépôt et à la diffusion de documents scientifiques de niveau recherche, publiés ou non, émanant des établissements d'enseignement et de recherche français ou étrangers, des laboratoires publics ou privés.

Published by Copernicus Publications on behalf of the European Geosciences Union. R. A. Zaveri et al.: Overview of the 2010 CARESAbstract. Substantial uncertainties still exist in the scientific understanding of the possible interactions between urban and natural (biogenic) emissions in the production and transformation of atmospheric aerosol and the resulting impact on climate change. The US Department of Energy (DOE) Atmospheric Radiation Measurement (ARM) program's Carbonaceous Aerosol and Radiative Effects Study (CARES) carried out in June 2010 in Central Valley, California, was a comprehensive effort designed to improve this understanding. The primary objective of the field study was to investigate the evolution of secondary organic and black carbon aerosols and their climate-related properties in the Sacramento urban plume as it was routinely transported into the forested Sierra Nevada foothills area. Urban aerosols and trace gases experienced significant physical and chemical transformations as they mixed with the reactive biogenic hydrocarbons emitted from the forest. Two heavily-instrumented ground sites -one within the Sacramento urban area and another about 40 km to the northeast in the foothills area -were set up to characterize the evolution of meteorological variables, trace gases, aerosol precursors, aerosol size, composition, and climaterelated properties in freshly polluted and "aged" urban air. On selected days, the DOE G-1 aircraft was deployed to make similar measurements upwind and across the evolving Sacramento plume in the morning and again in the afternoon. The NASA B-200 aircraft, carrying remote sensing instruments, was also deployed to characterize the vertical and horizontal distribution of aerosols and aerosol optical properties within and around the plume. This overview provides: (a) the scientific background and motivation for the study, (b) the operational and logistical information pertinent to the execution of the study, (c) an overview of key observations and initial findings from the aircraft and ground-based sampling platforms, and (d) a roadmap of planned data analyses and focused modeling efforts that will facilitate the integration of new knowledge into improved representations of key aerosol processes and properties in climate models.

The National Oceanic and Atmospheric Administration/Earth System Research Laboratory/Chemical Sciences Division (NOAA/ESRL/CSD) has developed a versatile, airborne lidar system for measuring ozone and aerosols in the boundary layer and lower free troposphere. The Tunable Optical Profiler for Aerosol and Ozone (TOPAZ) lidar was deployed aboard a NOAA Twin Otter aircraft during the Texas Air Quality Study (TexAQS 2006) and the California Research at the Nexus of Air Quality and Climate Change (CalNex 2010) field campaigns. TOPAZ is capable of measuring ozone concentrations in the lower troposphere with uncertainties of several parts per billion by volume at 90-m vertical and 600-m horizontal resolution from an aircraft flying at 60 m s−1. The system also provides uncalibrated aerosol backscatter profiles at 18-m vertical and 600-m horizontal resolution. TOPAZ incorporates state-of-the-art technologies, including a cerium-doped lithium calcium aluminum fluoride (Ce:LiCAF) laser, to make it compact and lightweight with low power consumption. The tunable, three-wavelength UV laser source makes it possible to optimize the wavelengths for differing atmospheric conditions, reduce the interference from other atmospheric constituents, and implement advanced analysis techniques. This paper describes the TOPAZ lidar, its components and performance during testing and field operation, and the data analysis procedure, including a discussion of error sources. The performance characteristics are illustrated through a comparison between TOPAZ and an ozonesonde launched during the TexAQS 2006 field campaign. A more comprehensive set of comparisons with in situ measurements during TexAQS 2006 and an assessment of the TOPAZ accuracy and precision are presented in a companion paper.