Surface plasmonic with its unique confinement of light is expected to be a cornerstone for future compact radiation sources and integrated photonics devices. The energy transfer between light and matter is a defining aspect that underlies recent studies on optical surface-wave-mediated spontaneous emissions. But coherent stimulated emission, being omnipresent in every laser system, remains to be realized and revealed in the optical near fields unambiguously and dynamically. Here, we present the coherent amplification of Terahertz surface plasmon polaritons via free electron stimulated emission. We demonstrate the evolutionary amplification process with a frequency redshift and lasts over 1-mm interaction length. The complementary theoretical analysis predicts a 100-order surface wave growth when a properly phase-matched electron bunch is used, which lays the ground for a stimulated surface wave light source and may facilitate capable means for matter manipulation, especially in the Terahertz band.

Compressing high-energy laser pulses to a single-cycle and realizing the “λ3 laser concept”, where λ is the wavelength of the laser, will break the current limitation of super-scale projects and contribute to the future 100-petawatt and even Exawatt lasers. Here, we have realized ultra-broadband gold gratings, core optics in the chirped pulse amplification, in the 750–1150 nm spectral range with a > 90% −1 order diffraction efficiency for near single-cycle pulse stretching and compression. The grating is also compatible with azimuthal angles from −15° to 15°, making it possible to design a three-dimensional compressor. In developing and manufacturing processes, a crucial grating profile with large base width and sharp ridge is carefully optimized and controlled to dramatically broaden the high diffraction efficiency bandwidth from the current 100–200 nm to over 400 nm. This work has removed a key obstacle to achieving the near single-cycle 100-PW lasers in the future.