There is strong circumstantial evidence that the shape of atomic nuclei with particular values of Z and N prefers to assume octupole deformation, in which the nucleus is distorted into a pear shape that loses the reflection symmetry of a quadrupole-deformed (rugby ball) shape prevalent in nuclei. Recently, useable intensities of accelerated beams of heavy, radioactive ions have become available at the REX-ISOLDE facility at CERN. This has allowed electric octupole transition strengths, a direct measure of octupole correlations, to be determined for short-lived isotopes of radon and radium expected to be unstable to pear-like distortions. The data are used to discriminate differing theoretical approaches to the description of the octupole phenomena, and also help restrict the choice of candidates for studies of atomic electric-dipole moments, that provide stringent tests of extensions to the Standard Model.

Abstract. The Miniball germanium detector array has been operational at the REX (Radioactive ion beam EXperiment) post accelerator at the Isotope Separator On-Line facility ISOLDE at CERN since 2001. During the last decade, a series of successful Coulomb excitation and transfer reaction studies have been performed with this array, utilizing the unique and high-quality radioactive ion beams which are available at ISOLDE. In this article, an overview is given of the technical details of the full Miniball setup, including a description of the γ-ray and particle detectors, beam monitoring devices and methods to deal with beam contamination. The specific timing properties of the REX-ISOLDE facility are highlighted to indicate the sensitivity that can be achieved with the full Miniball setup. The article is finalized with a summary of some physics highlights at REX-ISOLDE and the utilization of the Miniball germanium detectors at other facilities.

Coulomb-excitation experiments are performed with postaccelerated beams of neutron-deficient Po196,198,200,202 isotopes at the REX-ISOLDE facility. A set of matrix elements, coupling the low-lying states in these isotopes, is extracted. In the two heaviest isotopes, Po200,202, the transitional and diagonal matrix elements of the 2+1 state are determined. In Po196,198 multistep Coulomb excitation is observed, populating the 4+1,0+2, and 2+2 states. The experimental results are compared to the results from the measurement of mean-square charge radii in polonium isotopes, confirming the onset of deformation from Po196 onwards. Three model descriptions are used to compare to the data. Calculations with the beyond-mean-field model, the interacting boson model, and the general Bohr Hamiltonian model show partial agreement with the experimental data. Finally, calculations with a phenomenological two-level mixing model hint at the mixing of a spherical structure with a weakly deformed rotational structure.We acknowledge the support of the ISOLDE Collaboration and technical teams and, especially, the support of RILIS and REX. This work was supported by FWO-Vlaanderen (Belgium), by GOA/2010/010 (BOF KU Leuven), by the Interuniversity Attraction Poles Programme initiated by the Belgian Science Policy Office (BriX network P7/12), by the European Commission within the Seventh Framework Programme through I3-ENSAR (Contract No. RII3-CT-2010-262010), by the German BMBF under Contract Nos. 05P12PKFNE, 06DA9036I 05P12RDCIA, and 05P12RDCIB, by the UK Science and Technology Facilities Council, by the Spanish MINECO under Project No. FIS2011-28738-C02-02, by Narodowe Centrum Nauki (Polish Center for Scientific Research) Grant No. UMO-2013/10/M/ST2/00427, by the Academy of Finland (Contract No. 131665), and by the European Commission through the Marie Curie Actions call PIEFGA-2008-219174 (J.P.)

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A low-lying state in 131 In 82 , the one-proton hole nucleus with respect to double magic 132 Sn, was observed by its γ decay to the I π ¼ 1=2 − β-emitting isomer. We identify the new state at an excitation energy of E x ¼ 1353 keV, which was populated both in the β decay of 131 Cd 83 and after β-delayed neutron emission from 132 Cd 84 , as the previously unknown πp 3=2 single-hole state with respect to the 132 Sn core. Exploiting this crucial new experimental information, shell-model calculations were performed to study the structure of experimentally inaccessible N ¼ 82 isotones below 132 Sn. The results evidence a surprising absence of proton subshell closures along the chain of N ¼ 82 isotones. The consequences of this finding for the evolution of the N ¼ 82 shell gap along the r-process path are discussed.