A new summation method model of the reactor antineutrino energy spectrum is presented. It is updated with the most recent evaluated decay databases and with our Total Absorption Gammaray Spectroscopy measurements performed during the last decade. For the first time the spectral measurements from the Daya Bay experiment are compared with the detected antineutrino energy spectrum computed with the updated summation method without any renormalisation. The results exhibit a better agreement than is obtained with the Huber-Mueller model in the 2 to 5 MeV range, the region which dominates the detected flux. An unexpected systematic trend is found that the detected antineutrino flux computed with the summation model decreases with the inclusion of more Pandemonium free data. The detected flux obtained now lies only 1.9% above that detected in the Daya Bay experiment, a value that may be reduced with forthcoming new Pandemonium free data leaving less and less room to the reactor anomaly. Eventually, the new predictions of individual antineutrino spectra for the 235 U, 239 Pu, 241 Pu and 238 U are used to compute the dependence of the reactor antineutrino spectral shape on the fission fractions.
The β-delayed neutron emission probabilities of neutron rich Hg and Tl nuclei have been measured together with β-decay half-lives for 20 isotopes of Au, Hg, Tl, Pb, and Bi in the mass region N≳126. These are the heaviest species where neutron emission has been observed so far. These measurements provide key information to evaluate the performance of nuclear microscopic and phenomenological models in reproducing the high-energy part of the β-decay strength distribution. This provides important constraints on global theoretical models currently used in r-process nucleosynthesis.
The antineutrino spectra measured in recent experiments at reactors are inconsistent with calculations based on the conversion of integral beta spectra recorded at the ILL reactor. 92 Rb makes the dominant contribution to the reactor antineutrino spectrum in the 5-8 MeV range but its decay properties are in question. We have studied 92 Rb decay with total absorption spectroscopy. Previously unobserved beta feeding was seen in the 4.5-5.5 region and the GS to GS feeding was found to be 87.5(25)%. The impact on the reactor antineutrino spectra calculated with the summation method is shown and discussed.
Total absorption γ-ray spectroscopy of the β-delayed neutron emitters ^{87}Br, ^{88}Br, and ^{94}Rb We investigate the decay of 87,88 Br and 94 Rb using total absorption γ-ray spectroscopy. These important fission products are β-delayed neutron emitters. Our data show considerable βγ-intensity, so far unobserved in high-resolution γ-ray spectroscopy, from states at high excitation energy. We also find significant differences with the β intensity that can be deduced from existing measurements of the β spectrum. We evaluate the impact of the present data on reactor decay heat using summation calculations. Although the effect is relatively small it helps to reduce the discrepancy between calculations and integral measurements of the photon component for 235 U fission at cooling times in the range 1 − 100 s. We also use summation calculations to evaluate the impact of present data on reactor antineutrino spectra. We find a significant effect at antineutrino energies in the range of 5 to 9 MeV. In addition, we observe an unexpected strong probability for γ emission from neutron unbound states populated in the daughter nucleus. The γ branching is compared to Hauser-Feshbach calculations which allow one to explain the large value for bromine isotopes as due to nuclear structure. However the branching for 94 Rb, although much smaller, hints of the need to increase the radiative width Γγ by one order-of-magnitude. This increase in Γγ would lead to a similar increase in the calculated (n, γ) cross section for this very neutron-rich nucleus with a potential impact on r process abundance calculations.
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