We report results of a new technique to measure the electric dipole moment of 129 Xe with 3 He comagnetometry. Both species are polarized using spin-exchange optical pumping, transferred to a measurement cell, and transported into a magnetically shielded room, where SQUID magnetometers detect free precession in applied electric and magnetic fields. The result from a one week measurement campaign in 2017 and a 2.5 week campaign in 2018, combined with detailed study of systematic effects, is dA( 129 Xe) = (1.4 ± 6.6stat ± 2.0syst) × 10 −28 e cm. This corresponds to an upper limit of |dA( 129 Xe)| < 1.4 × 10 −27 e cm (95% CL), a factor of five more sensitive than the limit set in 2001.Searches for permanent electric dipole moments (EDMs) are a powerful way to investigate beyondstandard-model (BSM) physics. An EDM is a charge asymmetry along the total angular momentum axis of a particle or system and is odd under both parity reversal (P) and time reversal (T). Assuming CPT conservation (C is charge conjugation), an EDM is a direct signal of CP violation (CPV), a condition required to generate the observed baryon asymmetry of the universe [1]. The Standard Model incorporates CPV through the phase in the CKM matrix and the QCD parameterθ. However, the Standard Model alone is insufficient to explain the size of the baryon asymmetry [2]. BSM scenarios that generate the observed baryon asymmetry [3] generally also provide for EDMs larger than the SM estimate, which for 129 Xe is |d A ( 129 Xe) SM | ≈ 5 × 10 −35 e cm [4].EDM measurements have provided constraints on how BSM CPV can enter low-energy physics [4]. Diamagnetic systems such as 129 Xe and 199 Hg are particularly sensitive to CPV nucleon-nucleon interactions that induce a nuclear Schiff moment and CPV semileptonic couplings [7]. While the most precise atomic EDM measurement is from 199 Hg [8], there are theoretical challenges to constraining hadronic CPV parameters from 199 Hg alone, and improved sensitivity to the 129 Xe EDM would tighten these constraints [7,9]. Additionally, recent work has shown that contributions from light-axion-induced CPV are significantly stronger for 129 Xe than for 199

A versatile and portable magnetically shielded room with a field of (700 ± 200) pT within a central volume of 1 m × 1 m × 1 m and a field gradient less than 300 pT/m, achieved without any external field stabilization or compensation, is described. This performance represents more than a hundredfold improvement of the state of the art for a two-layer magnetic shield and provides an environment suitable for a next generation of precision experiments in fundamental physics at low energies; in particular, searches for electric dipole moments of fundamental systems and tests of Lorentz-invariance based on spin-precession experiments. Studies of the residual fields and their sources enable improved design of future ultra-low gradient environments and experimental apparatus. This has implications for developments of magnetometry beyond the femto-Tesla scale in, for example, biomagnetism, geosciences, and security applications and in general low-field nuclear magnetic resonance (NMR) measurements.

An increasing number of measurements in fundamental and applied physics rely on magnetically shielded environments with sub nano-Tesla residual magnetic fields. State of the art magnetically shielded rooms (MSRs) consist of up to seven layers of high permeability materials in combination with highly conductive shields. Proper magnetic equilibration is crucial to obtain such low magnetic fields with small gradients in any MSR. Here we report on a scheme to magnetically equilibrate MSRs with a 10 times reduced duration of the magnetic equilibration sequence and a significantly lower magnetic field with improved homogeneity. For the search of the neutron's electric dipole moment, our finding corresponds to a linear improvement in the systematic reach and a 40 % improvement of the statistical reach of the measurement. However, this versatile procedure can improve the performance of any MSR for any application.Comment: 5 pages, 4 figure

We present a magnetically shielded environment with a damping factor larger than one million at the mHz frequency regime and an extremely low field and gradient over an extended volume. This extraordinary shielding performance represents an improvement of the state-of-the-art in the difficult regime of damping very low-frequency distortions by more than an order of magnitude. This technology enables a new generation of high-precision measurements in fundamental physics and metrology, including searches for new physics far beyond the reach of accelerator-based experiments. We discuss the technical realization of the shield with its improvements in design.