[1] Updates for the Coupled Ocean-Atmosphere Response Experiment (COARE) physically based meteorological and gas transfer bulk flux algorithms are examined. The current versions are summarized and a generalization of the gas transfer codes to 79 gases is described. The current meteorological version COARE3.0 was compared with a collection of 26,700 covariance observations of drag and heat transfer coefficients (compiled from three independent research groups). The algorithm agreed on average to within 5% with observations for a wind speed range of 2 to 18 m s −1 . Covariance observations of CO 2 and dimethyl sulfide (DMS) gas transfer velocity k were normalized to Schmidt number 660 and compared to an ensemble of gas flux observations from six research groups and nine field programs. A reasonable fit of the mean k 660 versus U 10n values was obtained for both CO 2 and DMS with a new version of the COARE gas transfer algorithm (designated COAREG3.1) using friction velocity associated with viscous (tangential) stress, u * n , in the nonbubble term. In the wind speed range 5 to 16 m s , tracer-derived estimates of k 660 are 10% to 20% lower than the CO 2 covariance estimates presented here.

[1] Direct measurements of air-sea heat, momentum, and mass (including CO 2 , DMS, and water vapor) fluxes using the direct covariance method were made over the open ocean from the NOAA R/V Ronald H. Brown during the Southern Ocean Gas Exchange (SO GasEx) program. Observations of fluxes and the physical processes associated with driving air-sea exchange are key components of SO GasEx. This paper focuses on the exchange of CO 2 and the wind speed dependency of the transfer velocity, k, used to model the CO 2 flux between the atmosphere and ocean. A quadratic dependence of k on wind speed based on dual tracer experiments is most frequently encountered in the literature. However, in recent years, bubble-mediated enhancement of k, which exhibits a cubic relationship with wind speed, has emerged as a key issue for flux parameterization in high-wind regions. Therefore, a major question addressed in SO GasEx is whether the transfer velocities obey a quadratic or cubic relationship with wind speed. After significant correction to the flux estimates (primarily due to moisture contamination), the direct covariance CO 2 fluxes confirm a significant enhancement of the transfer velocity at high winds compared with previous quadratic formulations. Regression analysis suggests that a cubic relationship provides a more accurate parameterization over a wind speed range of 0 to 18 m s −1 . The Southern Ocean results are in good agreement with the 1998 GasEx experiment in the North Atlantic and a recent separate field program in the North Sea.

Abstract. The Atlantic Tradewind Ocean-Atmosphere Mesoscale Interaction Campaign (ATOMIC) took place from 7 January to 11 July 2020 in the tropical North Atlantic between the eastern edge of Barbados and 51∘ W, the longitude of the Northwest Tropical Atlantic Station (NTAS) mooring. Measurements were made to gather information on shallow atmospheric convection, the effects of aerosols and clouds on the ocean surface energy budget, and mesoscale oceanic processes. Multiple platforms were deployed during ATOMIC including the NOAA RV Ronald H. Brown (RHB) (7 January to 13 February) and WP-3D Orion (P-3) aircraft (17 January to 10 February), the University of Colorado's Robust Autonomous Aerial Vehicle-Endurant Nimble (RAAVEN) uncrewed aerial system (UAS) (24 January to 15 February), NOAA- and NASA-sponsored Saildrones (12 January to 11 July), and Surface Velocity Program Salinity (SVPS) surface ocean drifters (23 January to 29 April). The RV Ronald H. Brown conducted in situ and remote sensing measurements of oceanic and atmospheric properties with an emphasis on mesoscale oceanic–atmospheric coupling and aerosol–cloud interactions. In addition, the ship served as a launching pad for Wave Gliders, Surface Wave Instrument Floats with Tracking (SWIFTs), and radiosondes. Details of measurements made from the RV Ronald H. Brown, ship-deployed assets, and other platforms closely coordinated with the ship during ATOMIC are provided here. These platforms include Saildrone 1064 and the RAAVEN UAS as well as the Barbados Cloud Observatory (BCO) and Barbados Atmospheric Chemistry Observatory (BACO). Inter-platform comparisons are presented to assess consistency in the data sets. Data sets from the RV Ronald H. Brown and deployed assets have been quality controlled and are publicly available at NOAA's National Centers for Environmental Information (NCEI) data archive (https://www.ncei.noaa.gov/archive/accession/ATOMIC-2020, last access: 2 April 2021). Point-of-contact information and links to individual data sets with digital object identifiers (DOIs) are provided herein.

Abstract. The Atlantic Tradewind Ocean-Atmosphere Mesoscale Interaction Campaign (ATOMIC), part of the larger experiment known as Elucidating the Role of Clouds-Circulation Coupling in Climate (EUREC4A), was held in the western Atlantic during the period 17 January–11 February 2020. This paper describes observations made during ATOMIC by the US National Oceanic and Atmospheric Administration's (NOAA) Lockheed WP-3D Orion research aircraft based on the island of Barbados. The aircraft obtained 95 h of observations over 11 flights, many of which were coordinated with the NOAA research ship R/V Ronald H. Brown and autonomous platforms deployed from the ship. Each flight contained a mixture of sampling strategies including high-altitude circles with frequent dropsonde deployment to characterize the large-scale environment, slow descents and ascents to measure the distribution of water vapor and its isotopic composition, stacked legs aimed at sampling the microphysical and thermodynamic state of the boundary layer, and offset straight flight legs for observing clouds and the ocean surface with remote sensing instruments and the thermal structure of the ocean with in situ sensors dropped from the plane. The characteristics of the in situ observations, expendable devices, and remote sensing instrumentation are described, as is the processing used in deriving estimates of physical quantities. Data archived at the National Center for Environmental Information include flight-level data such as aircraft navigation and basic thermodynamic information (NOAA Aircraft Operations Center and NOAA Physical Sciences Laboratory, 2020, https://doi.org/10.25921/7jf5-wv54); high-accuracy measurements of water vapor concentration from an isotope analyzer (National Center for Atmospheric Research, 2020, https://doi.org/10.25921/c5yx-7w29); in situ observations of aerosol, cloud, and precipitation size distributions (Leandro and Chuang, 2020, https://doi.org/10.25921/vwvq-5015); profiles of seawater temperature made with Airborne eXpendable BathyThermographs (AXBTs; NOAA Physical Sciences Laboratory, 2020a, https://doi.org/10.25921/pe39-sx75); radar reflectivity, Doppler velocity, and spectrum width from a nadir-looking W-band radar (NOAA Physical Sciences Laboratory, 2020c, https://doi.org/10.25921/n1hc-dc30); estimates of cloud presence, the cloud-top location, and the cloud-top radar reflectivity and temperature, along with estimates of 10 m wind speed obtained from remote sensing instruments operating in the microwave and thermal infrared spectral regions (NOAA Physical Sciences Laboratory, 2020b, https://doi.org/10.25921/x9q5-9745); and ocean surface wave characteristics from a Wide Swath Radar Altimeter (Prosensing, Inc., 2020, https://doi.org/10.25921/qm06-qx04). Data are provided as netCDF files following Climate and Forecast conventions.

Abstract. The Atlantic Tradewind Ocean-Atmosphere Mesoscale Interaction Campaign (ATOMIC) took place from January 7 to July 11, 2020 in the tropical North Atlantic between the eastern edge of Barbados and 51° W, the longitude of the Northwest Tropical Atlantic Station (NTAS) mooring. Measurements were made to gather information on shallow atmospheric convection, the effects of aerosols and clouds on the ocean surface energy budget, and mesoscale oceanic processes. Multiple platforms were deployed during ATOMIC including the NOAA RV Ronald H. Brown (RHB) (Jan. 7 to Feb. 13) and WP-3D Orion (P-3) aircraft (Jan. 17 to Feb. 10), the University of Colorado's RAAVEN Uncrewed Aerial System (UAS) (Jan. 24 to Feb. 15), NOAA- and NASA-sponsored Saildrones (Jan. 12 to Jul. 11), and Surface Velocity Program Salinity (SVPS) surface ocean drifters (Jan. 23 to Apr. 29). The RV Ronald H. Brown conducted in situ and remote sensing measurements of oceanic and atmospheric properties with an emphasis on mesoscale oceanic-atmospheric coupling and aerosol-cloud interactions. In addition, the ship served as a launching pad for Wave Gliders, Surface Wave Instrument Floats with Tracking (SWIFTs), and radiosondes. Details of measurements made from the RV Ronald H. Brown, ship-deployed assets, and other platforms closely coordinated with the ship during ATOMIC are provided here. These platforms include Saildrone 1064 and the RAAVEN UAS as well as the Barbados Cloud Observatory (BCO) and Barbados Atmospheric Chemistry Observatory (BACO). Inter-platform comparisons are presented to assess consistency in the data sets. Data sets from the RV Ronald H. Brown and deployed assets have been quality controlled and are publicly available at the NOAA Physical Sciences Laboratory (PSL) ATOMIC ftp server (ftp://ftp2.psl.noaa.gov/Projects/ATOMIC/data/ (Quinn et al., 2020). In addition, the data have been submitted to NOAA's National Centers for Environmental Information (NCEI) data archive (https://www.ncei.noaa.gov/) for Digital Object Identifiers (DOIs). Point of contact information and links to individual data sets are provided herein.