Flexible pressure sensors with high sensitivity over a broad pressure range are highly desired, yet challenging to build to meet the requirements of practical applications in daily activities and more significant in some extreme environments. This work demonstrates a thin, lightweight, and high-performance pressure sensor based on flexible porous phenyl-silicone/functionalized carbon nanotube (PS/FCNT) film. The formed crack-across-pore endows the pressure sensor with high sensitivity of 19.77 kPa–1 and 1.6 kPa–1 in the linear range of 0–33 kPa and 0.2–2 MPa, respectively, as well as ultralow detection limit (∼1.3 Pa). Furthermore, the resulting pressure sensor possesses a low fatigue over 4000 loading/unloading cycles even under a high pressure of 2 MPa and excellent durability (>6000 cycles) after heating at high temperature (200 °C), attributed to the strong chemical bonding between PS and FCNT, excellent mechanical stability, and high temperature resistance of PS/FCNT film. These superior properties set a foundation for applying the single sensor device in detecting diverse stimuli from the very low to high pressure range, including weak airflow, sway, vibrations, biophysical signal monitoring, and even car pressure. Besides, a deep neural network based on transformer (TRM) has been engaged for human action recognition with an overall classification rate of 94.96% on six human actions, offering high accuracy in real-time practical scenarios.

Thin, lightweight, and flexible textile pressure sensors with the ability to detect the full range of faint pressure (<100 Pa), low pressure (≈KPa) and high pressure (≈MPa) are in significant demand to meet the requirements for applications in daily activities and more meaningfully in some harsh environments, such as high temperature and high pressure. However, it is still a significant challenge to fulfill these requirements simultaneously in a single pressure sensor. Herein, a high‐performance pressure sensor enabled by polyimide fiber fabric with functionalized carbon‐nanotube (PI/FCNT) is obtained via a facile electrophoretic deposition (EPD) approach. High‐density FCNT is evenly wrapped and chemically bonded to the fiber surface during the EPD process, forming a conductive hierarchical fiber/FCNT matrix. Benefiting from the large compressible region of PI fiber fabric, abundant yet firm contacting points and high elastic modulus of both PI and CNT, the proposed pressure sensor can be customized and modulated to achieve both an ultra‐broad sensing range, long‐term stability and high‐temperature resistance. Thanks to these merits, the proposed pressure sensor could monitor the human physiological information, detect tiny and extremely high pressure, can be integrated into an intelligent mechanical hand to detect the contact force under high‐temperature.