“…This was the case, for example, to assess the contributions of the Chernobyl fallout (Mitchell et al, 1990;Holm et al 1992;Pourcelot et al, 2003;Le Roux et al, 2010;Popov et al, 2010), or those of a nuclear industry (Charmasson et al, 1998;Duffa et al, 2001;Ueda et al, 2004;Gauthier-Lafaye et al, 2008). Mass spectrometry has been increasingly used in recent decades to supplement information; by having the advantage of direct access to accurate isotopic ratios, in particular with the atomic ratios of isotopes of heavy elements such as plutonium, to discern the local-regional fallout of a test site (Lindahl et al, 2011;Tims et al, 2016;Buessler et al, 2018;Huang et al, 2019). This applies especially to the ( 240 Pu/ 239 Pu) AR , whose values have been widely characterized for various types of installation, accident or use of nuclear material (Mitchell et al, 1997;Warneke et al, 2002;Eriksson et al, 2008;Lindhal et al, 2010).…”