2016
DOI: 10.1016/j.jenvrad.2015.06.020
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236U and 239,240Pu ratios from soils around an Australian nuclear weapons test site

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Cited by 34 publications
(8 citation statements)
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“…Numerous studies have confirmed that the radioactive substances contained in nuclear wastewater pose a great threat to the natural environment on which humans depend and to their own health (Clifford and Zhang 1994;Dufresne et al 2018). Normile (2021) stated that unlike other radioisotopes with significant risks, such as 131 I, 236 U, 240 P, 137 Cs (Tims et al 2016;Cléro et al 2021;Tsabaris et al 2021), the large amount of 3 H contained in nuclear wastewater from the FDNPP is more hazardous. Currently, approximately 1PBq 3 H is stored in storage tanks at FDNPP (de With et al 2021).…”
Section: Nuclear Wastewater Managementmentioning
confidence: 99%
“…Numerous studies have confirmed that the radioactive substances contained in nuclear wastewater pose a great threat to the natural environment on which humans depend and to their own health (Clifford and Zhang 1994;Dufresne et al 2018). Normile (2021) stated that unlike other radioisotopes with significant risks, such as 131 I, 236 U, 240 P, 137 Cs (Tims et al 2016;Cléro et al 2021;Tsabaris et al 2021), the large amount of 3 H contained in nuclear wastewater from the FDNPP is more hazardous. Currently, approximately 1PBq 3 H is stored in storage tanks at FDNPP (de With et al 2021).…”
Section: Nuclear Wastewater Managementmentioning
confidence: 99%
“…This was the case, for example, to assess the contributions of the Chernobyl fallout (Mitchell et al, 1990;Holm et al 1992;Pourcelot et al, 2003;Le Roux et al, 2010;Popov et al, 2010), or those of a nuclear industry (Charmasson et al, 1998;Duffa et al, 2001;Ueda et al, 2004;Gauthier-Lafaye et al, 2008). Mass spectrometry has been increasingly used in recent decades to supplement information; by having the advantage of direct access to accurate isotopic ratios, in particular with the atomic ratios of isotopes of heavy elements such as plutonium, to discern the local-regional fallout of a test site (Lindahl et al, 2011;Tims et al, 2016;Buessler et al, 2018;Huang et al, 2019). This applies especially to the ( 240 Pu/ 239 Pu) AR , whose values have been widely characterized for various types of installation, accident or use of nuclear material (Mitchell et al, 1997;Warneke et al, 2002;Eriksson et al, 2008;Lindhal et al, 2010).…”
Section: Introductionmentioning
confidence: 99%
“…By contrast, the link between a specific isotope, considered via the isotopic ratio, and its origin often yields a more tangible association 13 , for example: a pre-detonation weapon safety test might cause 239 Pu to dominate; fallout from atmospheric detonations can comprise higher-mass isotopes through to 244 Pu (refs. 14 , 15 ), whereas a relatively low 240 Pu/ 239 Pu ratio might reflect the low proportions of 240 Pu desirable in some applications, such as that obtained by breeding. Material dispersed in fallout will often have a higher proportion of 244 Pu (ref.…”
Section: Introductionmentioning
confidence: 99%