We report the frequency-dependent optical constants, n(ν) and R(ν), or, equivalently, the complex permittivity ˆ(ω) ) ′(ω)i ′′(ω), over the frequency range from 2 to 50 cm -1 for water, methanol, ethanol, 1-propanol, and liquid ammonia. These spectra have been measured with femtosecond terahertz pulse transmission spectroscopy. These liquids exhibit multiple-Debye behavior, making their frequency-dependent dielectric constants valuable benchmarks for molecular dynamics simulations and other theoretical treatments of liquids.