2021
DOI: 10.1029/2020jc017092
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A 30 ‐Year Time Series of Transient Tracer‐Based Estimates of Anthropogenic Carbon in the Central Labrador Sea

Abstract: The change in oceanic total dissolved inorganic carbon (DIC) concentrations relative to pre-industrial values, due to human mobilization of carbon over the past 250 years, is defined as "excess" or "anthropogenic" carbon dioxide (Excess CO 2 or C ant ; D. Wallace, 2001). This C ant represents only a small fraction of the total dissolved CO 2 , and therefore difficulties are encountered in distinguishing the anthropogenic perturbation from the predominant natural signal. This is further complicated by spatial a… Show more

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Cited by 12 publications
(18 citation statements)
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“…However, the CFC‐12 saturation is not constant and seems to increase with time (Figure S2 in Supporting Information ). This is in agreement with what has been found in the North Atlantic (Tanhua et al., 2008) and the Labrador Sea (Raimondi et al., 2021). This evolution is most clearly seen in the Greenland Sea, but also seems to be the case in the other basins.…”
Section: Methodssupporting
confidence: 93%
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“…However, the CFC‐12 saturation is not constant and seems to increase with time (Figure S2 in Supporting Information ). This is in agreement with what has been found in the North Atlantic (Tanhua et al., 2008) and the Labrador Sea (Raimondi et al., 2021). This evolution is most clearly seen in the Greenland Sea, but also seems to be the case in the other basins.…”
Section: Methodssupporting
confidence: 93%
“…This will have an impact on the calculated C ant concentrations. Changes in the disequilibrium have been found to translate almost linearly to the C ant values both in the Nordic Seas and the Labrador Sea (Olsen et al., 2010; Raimondi et al., 2021). Consequently, an ocean surface with a p CO 2 growth rate of 80% compared to the atmospheric p CO 2 , will reduce the C ant estimates by 20%.…”
Section: Methodsmentioning
confidence: 99%
“…However, an important caveat regarding our finding of a progressively weakening North Atlantic C ant sink is the fact that the available ocean interior observations in the North Atlantic stem mostly from the first half of our last sampling period, the 2010s. However, after 2013 the NAO switched to a strong positive phase (Holliday et al., 2020) and in line with this, the C ant column inventories in the Central Labrador Sea rapidly increased (Raimondi et al., 2021). Likewise, a deep convection event in the Irminger Sea in winter 2014/15 injected anthropogenic carbon into the ocean interior and almost tripled the storage rates compared to those determined from previous hydrographic sections (Fröb et al., 2016).…”
Section: Discussionmentioning
confidence: 77%
“…While all sampling periods assigned for this study are relatively well covered with observations, the large changes we reconstruct in the North Atlantic between the first and second period need to be viewed with caution since the number of data records that provide all required variables for the eMLR(C*) analysis is very limited after ∼2015. During this period, a reinvigoration of the anthropogenic carbon accumulation has been reported in regional studies (Fröb et al, 2018;Raimondi et al, 2021), albeit only for small subregions of the whole North Atlantic.…”
Section: Caveats and Recommendationsmentioning
confidence: 90%
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