Grattan, J.P., Gilbertson, D.D., Hunt, C.O. (2007). The local and global dimensions of metaliferrous air pollution derived from a reconstruction of an 8 thousand year record of copper smelting and mining at a desert-mountain frontier in southern Jordan. Journal of Archaeological Science 34, 83-110This paper establishes an eight thousand year history of anthropogenic metal pollution at one of the oldest, most important and longest sustained sites of the extraction and smelting of copper ores in the Old World: the Faynan Orefield in Jordan, which is located between the hyper-arid southern desert and the front of the wetter Mountains of Edom. The modern land surface is shown, in significant part, to be a complex palimpsest of archaeological sites, metal pollution of various ages and ore processing deposits. Quantitative and qualitative observations of the storage and cycling of heavy metals through the local natural and domestic systems have produced a body of information on processes with which the past has been interpreted. Heavy metal concentrations in semi-continuous sedimentary bodies indicate that over the last 1500years, metals were removed by natural processes at a comparatively slow rate given the scale of the original anthropogenic metal burden: the proportions of lead with respect to copper have increased as the overall metal burden has been lowered. Distinctive anthropogenic metal-pollution signatures have been detected in ash- and charcoal-rich deposits that were discarded onto the banks of a perennial stream in the late Neolithic. At present, the nature of the human activities that might have produced these pollution signatures is unknown. Substantial metal pollution from industrial-scale smelting activity was present from the Early Bronze Age. The intensity of heavy metal pollution produced in Classical Times locally exceeded that recorded at major European copper smelting centres in the nineteenth century A.D. The pollution evidence indicates that intensive copper smelting at the immediate area took place until approximately the end of the Byzantine period; with the exception of one further minor episode of smelting radiocarbon dated to cal. BP 530-330. An observed partial, but perhaps significant, parallelism is also noted between this local record and the records of the metal burdens of the northern hemisphere determined at mire or ice-sheet sites at high-altitudes or high-latitudes. The paper discusses the extent to which this parallelism might be a geochemical indicator of the actual existence of ''economic systems'' of a geographical scope and scale to have both exercised substantial ''pull'' upon the resources of such isolated and difficult locations at the Wadi Faynan, and to have generated sufficient overall metal pollution to have materially altered the chemistry of the global atmosphere. The comparative absence of quantitative information upon the nature, spatial scale and impacts of human, industrial and natural processes affecting metal-pollution in other metal-rich arid lands provides a ...
