This paper synthesizes and summarizes atmospheric variability on time scales from seconds to decades through a phenomenological census. We focus mainly on unforced variability in the troposphere, stratosphere, and mesosphere. In addition to atmosphere-only modes, our scope also includes coupled modes, in which the atmosphere interacts with the other components of the Earth system, such as the ocean, hydrosphere, and cryosphere. The topics covered include turbulence on time scales of seconds and minutes, gravity waves on time scales of hours, weather systems on time scales of days, atmospheric blocking on time scales of weeks, the Madden-Julian Oscillation on time scales of months, the Quasi-Biennial Oscillation and El Niño-Southern Oscillation on time scales of years, and the North Atlantic, Arctic, Antarctic, Pacific Decadal, and Atlantic Multidecadal Oscillations on time scales of decades. The paper serves as an introduction to a special collection of Geophysical Research Letters on atmospheric variability. We hope that both this paper and the collection will serve as a useful resource for the atmospheric science community and will act as inspiration for setting future research directions. the atmosphere interacts with the other components of the Earth system, such as the ocean, hydrosphere, and cryosphere. Given these interactions, and the importance of the atmosphere for weather and climate, our intended audience is the entire Geophysical Research Letters readership. Our aim is to provide an authoritative, concise, and accessible point of reference for the most important modes of atmospheric variability. This Commentary serves as an introductory foreword to a virtual special collection of Geophysical Research Letters on atmospheric variability. To initiate the collection, we have identified some of the most influential and definitive papers to have been published in this journal in recent years. Our hope and expectation is that this will be a living collection, which will grow over time whenever seminal new papers are published. The contents of the Commentary are ordered in terms of increasing time scale, from seconds and minutes (section 2), to hours (section 3), days (section 4), weeks (section 5), months (section 6), years (section 7), and decades (section 8). We note at the outset, however, that the time scales of many atmospheric phenomena are not unambiguously defined. For example, the Madden-Julian Oscillation (section 6) is monitored and WILLIAMS ET AL.