The development of artificial intelligence (AI) and Internet of things (IoT) technologies has resulted in a groundbreaking shift in urban connectivity that has enabled the creation of smart cities. This chapter looks at how AI-infused urban connections have greatly impacted the growth of IoT communication networks. By utilizing AI, smart cities can improve public services, improve the utilization of assets, and increase urban living standards. Important subjects covered in this chapter include predictive maintenance, real-time monitoring, and AI-driven data analytics, all of which increase the efficiency and dependability of urban infrastructure. The integration of IoT devices and AI algorithms in urban settings is examined in this chapter, featuring concerns including security, privacy, and regulatory frameworks being addressed. Through case studies and practical examples, it offers a thorough explanation of how AI-infused urban connectivity is redefining smart cities and encouraging the creation of next-generation IoT communication networks.