“…In past years, many Tm-Ho codoped laser crystals have been widely used to generate 2 µm lasers, such as Y 3 Al 5 O 12 (YAG), YAlO 3 (YAP), GdVO 4 , YVO 4 , YLiF 4 (YLF), and LuLiF 4 (LLF). [2][3][4][5]. Among these known Tm-Ho codoped materials, Tm,Ho:LLF is an excellent laser crystal due to the good thermo-optical and thermo-mechanical properties, high natural birefringence, low upconversion effect, and large energy spread of the manifolds [5,6].…”