“…6,9 The capture-release of water vapor has underpinned a number of emerging designs significant to the water-energy nexus, such as sorption-driven heat transformation for cooling and heating, [10][11][12][13][14] atmospheric water harvesting (AWH), [15][16][17][18][19][20][21][22][23][24][25][26][27][28] vapor-sorption-based desalination, 14,29 and air humidity regulation. 30,31 In particular, sorptiondriven cooling and AWH are gaining a lot of interest nowadays in both academia and industry as they aim at reducing electricity consumption, obsoleting the conventional harmful coolants (e.g., chlorodifluoromethane, 1,1,1,2-tetrafluoroethane), 32 and producing freshwater from an unconventional source (the atmosphere). In all of these applications, the water vapor sorbent is the most critical component.…”