The emerging type II Weyl semimetal 1T′ MoTe2 as a promising material in polarization-sensitive photodetectors
has aroused much attention due to its narrow bandgap and intrinsic
in-plane anisotropic crystal structure. However, the semimetal properties
lead to a large dark current and a low response. Herein, we demonstrate
for the first time an all-2D semimetal MoTe2/MoS2 van der Waals (vdWs) heterojunction to improve the performance of
the photodetectors and realize polarization-sensitive, self-powered,
and broadband photodetection and imaging. Owing to the built-in electric
field of the heterojunction, the device achieves a self-powered photoresponse
ranging from 520 to 1550 nm. Under 915 nm light illumination, the
device demonstrates outstanding performance, including a high responsivity
of 79 mA/W, a specific detectivity of 1.2 × 1010 Jones,
a fast rise/decay time of 180/202 μs, and a high on/off ratio
of 1.3 × 10.3 Wavelength-dependent photocurrent anisotropic
ratio is revealed to vary from 1.10 at 638 nm to 2.24 at 1550 nm.
Furthermore, we demonstrate the polarization imaging capabilities
of the device in scattering surroundings, and the DoLP and AoLP images
achieve 78% and 112% contrast enhancement, respectively, compared
to the S0. This work opens up new avenues to develop anisotropic
semimetals heterojunction photodetectors for high-performance polarization-sensitive
photodetection and next-generation polarized imaging.