The amalgamation of sustainable practises throughout the fabrication process with advanced material engineering holds promise not only for eco-conscious manufacturing but also for promoting technological advancements in versatile material design and application. Moreover, technological innovation serves as a catalyst for sustainability initiatives, driving innovation and enabling the adoption of greener practises across industries. This study investigates redefining the production protocol of pressure spinning to produce core–sheath polymer fibres, deepening sustainable practises. It aims to explore innovative approaches such as modifying spinning parameters, optimising polymer solvent configurations and understanding fluid behaviour to curtail material wastage and maintain minimal energy consumption without compromising production efficiency. Utilising Polyvinylpyrrolidone (PVP) for the core and Polyethylene oxide (PEO) for the sheath, production rates of up to 64 g/h were achieved with a fibre diameter range of 3.2 ± 1.7 µm to 4.6 ± 2.0 µm. Energy consumption per mass of fibres produced showed a decreasing trend overall with increasing applied gas pressure. These findings highlight the potential for the efficient and scalable production of core–sheath fibres with applications in various advanced materials fields.