A N-doped carbon-supported In2O3 catalyst for highly efficient CO2 electroreduction to HCOOH

Zhang, Jie; Liang, Manfen; Xu, Haimei; Huang, Hong; Meng, Jian; Mu, Jinglin; Miao, Zhichao; Zhou, Jin

doi:10.1039/d3cc05872g

Chem. Commun.

2024

DOI: 10.1039/d3cc05872g

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A N-doped carbon-supported In₂O₃ catalyst for highly efficient CO₂ electroreduction to HCOOH

Jie Zhang,

Manfen Liang,

Haimei Xu

et al.

Abstract: The synergistic promotion of C and N species successfully enhances the activity of an In2O3@NC catalyst in CO2 electroreduction to HCOOH.

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Cited by 4 publications

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Theoretical Prediction Leads to Synthesize GDY Supported InO_x Quantum Dots for CO₂ Reduction

He,

Chen,

Xue

et al. 2024

Angewandte Chemie

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The preparation of formic acid by direct reduction of carbon dioxide is an important basis for the future chemical industry and is of great significance. Due to the serious shortage of highly active and selective electrocatalysts leading to the development of direct reduction of carbon dioxide is limited. Herein the target catalysts with high CO2RR activity and selectivity were identified by integrating DFT calculations and high‐throughput screening and by using graphdiyne (GDY) supported metal oxides quantum dots (QDs) as the ideal model. It is theoretically predicted that GDY supported indium oxide QDs (i.e., InOx/GDY) is a new heterostructure electrocatalyst candidate with optimal CO2RR performance. The interfacial electronic strong interactions effectively regulate the surface charge distribution of QDs and affect the adsorption/desorption behavior of HCOO* intermediate during CO2RR to achieve highly efficient CO2 conversion. Based on the predicted composition and structure, we synthesized the advanced catalytic system, and demonstrates superior CO2‐to‐HCOOH conversion performance. The study presents an effective strategy for rational design of highly efficient heterostructure electrocatalysts to promote green chemical production.

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Theoretical Prediction Leads to Synthesize GDY Supported InO_x Quantum Dots for CO₂ Reduction

He,

Chen,

Xue

et al. 2024

Angewandte Chemie

View full text Add to dashboard Cite

show abstract

Theoretical Prediction Leads to Synthesize GDY Supported InO_x Quantum Dots for CO₂ Reduction

He,

Chen,

Xue

et al. 2024

Angew Chem Int Ed

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Regulating p-orbital electronic configuration of In2O3 by thickness-controlled carbon layer for efficient electrocatalytic CO2 reduction to HCOOH

Meng,

Liang,

et al. 2025

Applied Catalysis B: Environment and Energy

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A N-doped carbon-supported In₂O₃ catalyst for highly efficient CO₂ electroreduction to HCOOH

Abstract: The synergistic promotion of C and N species successfully enhances the activity of an In2O3@NC catalyst in CO2 electroreduction to HCOOH.

Cited by 4 publications

References 17 publications

Theoretical Prediction Leads to Synthesize GDY Supported InO_x Quantum Dots for CO₂ Reduction

Theoretical Prediction Leads to Synthesize GDY Supported InO_x Quantum Dots for CO₂ Reduction

Theoretical Prediction Leads to Synthesize GDY Supported InO_x Quantum Dots for CO₂ Reduction

Regulating p-orbital electronic configuration of In2O3 by thickness-controlled carbon layer for efficient electrocatalytic CO2 reduction to HCOOH

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A N-doped carbon-supported In2O3 catalyst for highly efficient CO2 electroreduction to HCOOH

Abstract: The synergistic promotion of C and N species successfully enhances the activity of an In2O3@NC catalyst in CO2 electroreduction to HCOOH.

Cited by 4 publications

References 17 publications

Theoretical Prediction Leads to Synthesize GDY Supported InOx Quantum Dots for CO2 Reduction

Theoretical Prediction Leads to Synthesize GDY Supported InOx Quantum Dots for CO2 Reduction

Theoretical Prediction Leads to Synthesize GDY Supported InOx Quantum Dots for CO2 Reduction

Regulating p-orbital electronic configuration of In2O3 by thickness-controlled carbon layer for efficient electrocatalytic CO2 reduction to HCOOH

Contact Info

Product

Resources

About

A N-doped carbon-supported In₂O₃ catalyst for highly efficient CO₂ electroreduction to HCOOH

Theoretical Prediction Leads to Synthesize GDY Supported InO_x Quantum Dots for CO₂ Reduction

Theoretical Prediction Leads to Synthesize GDY Supported InO_x Quantum Dots for CO₂ Reduction

Theoretical Prediction Leads to Synthesize GDY Supported InO_x Quantum Dots for CO₂ Reduction