As an emerging candidate for a sustainable power supply,
moisture-electric
generators (MEGs) have attracted great attention in recent years.
Unlike the conventional hydroelectric system, MEGs propose to harvest
energy from ambient moisture, driven by either ion diffusion under
a concentration gradient or the interaction between a solid–liquid
interface governed by electrostatic theory. Two-dimensional (2D) nanomaterials,
in particular hydrophilic graphene oxide (GO), have been considered
as the most promising materials for high-performance MEGs owing to
their unique structure and properties. In line with the development
of 2D nanomaterials, the recent electrical output of a single MEG
has been greatly raised from tens to hundreds of millivolts, which
is capable of powering commercial electronics. Herein, we have reviewed
the recent progress of 2D nanomaterials in MEGs. The mechanism of
moisture-induced electricity generation and strategies for tailoring
2D nanomaterials to enhance the output performance of MEGs are discussed.
The potential application of MEGs is also discussed in two categories:
sensing and power supply. Finally, the existing challenges and the
perspective of MEGs are proposed for future study.