A novel designed 3D multi-microhole plasma jet device driven by nanosecond pulse at atmospheric pressure

Abstract

A novel designed three-dimensional (3D) multi-microhole helium plasma jet device excited by nanosecond pulse is developed in atmospheric air. Systematical investigations about the discharge characteristics are carried out to get insights into the formation mechanisms of 3D plasma jets. Results show that the 3D plasma jets originated from the branching of a single ionization wave to present a hexagonal-like structure including bottom jet (BJ) and side jets (SJ1 and SJ2). The BJ always keeps a stable performance while the SJ displays a remarkably turbulent mode. The dynamic evolution, and the propagation velocity and distance for BJ and SJ demonstrate significant differences, with a delay effect between BJ and SJ bullets propagation being observed. The OES show that 3D jets possess a high yield of the spatial distribution of reactive species in jet plumes. The formation mechanism of 3D jets is determined by the hydrodynamic (He flow distribution) and electrical interactions (distribution of electric field force) in the discharge tube emerging from individual holes with different radial directions. The direct treatment of water using this developed underwater 3D plasma device results in the production of plasma activated water (PAW) with a lower pH value, higher conductivity, and greater concentrations of reactive oxygen and nitrogen species (RONS), compared to the indirect treatment. Especially, the concentration of H2O2 can remarkably increase 141 folds from 1.43 to 202.12 μM within 5 mins after the direct 3D plasma treatment. This novel-designed 3D jets-based technique is a promising platform for 3D application scenarios, especially in the case of underwater microbubble discharge, which is of great significance for water activation in emerging applications.

Temporal evolution characteristics of the excited species in a pulsed needle-water discharge: effect of voltage and frequency

“…Atmospheric pressure non-thermal plasmas have expressed broad prospects in many fields because of their remarkable chemical activity achieved at a gas temperature near room temperature [1][2][3][4][5]. In some specific areas such as water purification and plasma activated water preparation, the plasmas inevitably come into contact with the liquid [6][7][8][9][10].…”

The addition of hydrogen peroxide and the incorporation of fluorides by surface plasma jointly promote the bactericidal effects of plasma-treated water

“…The pH value of PTH was 2.69 after treatment by the plasma for 4 min, demonstrating an increase of H + concentration by several orders of magnitude. However, OH was not detected in PTH, possibly because of the extremely low concentration with the configuration for indirect plasma treatment of water [40]. Also, the concentration of O 3 cannot be precisely measured in our experiments due to that some other reactive species, such as superoxide, could bleach the indigo reagent for detecting O 3 [41].…”

Insights into reactivity and bactericidal effects of water activated by He and Ar plasma jets

“…N 2 + (B) could be attributed to the Penning effect between metastable He species and N 2 , and O(3p 5p ) is mainly from the oxygen in air colliding with excited He species. [ 17 ] Additionally, the unique peaks of excited He* (at 706 nm) and excited Ar* (range from 700 to 800 nm) are tested in the He and Ar plasma jet, respectively.…”