A photochromic metal–organic framework with a rare 3D self-interpenetrated architecture and an ultrahigh MnO<sub>4</sub><sup>−</sup> sensing ability

Zhang, Jinfang; Yue, Yinlong; Tao, Xingyu; Zhang, Jiarun; Yin, Dejing; Zhang, Chi

doi:10.1039/d4nj02133a

New J. Chem.

2024

DOI: 10.1039/d4nj02133a

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A photochromic metal–organic framework with a rare 3D self-interpenetrated architecture and an ultrahigh MnO₄⁻ sensing ability

Jinfang Zhang,

Yinlong Yue,

Xingyu Tao

et al.

Abstract: Photochromic materials have shown a wide range of applications.

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Cited by 2 publications

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Pyridyl/Pyrimidyl-Containing Ligands Modulating Two Cd(II)-MOFs with Distinct Architectures and Al³⁺ Sensing Abilities

Zhang,

Yue,

Lin

et al. 2024

Inorg. Chem.

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It is a challenging task to develop metal−organic frameworks (MOFs) with fascinating architectures and outstanding performance. In this work, two novel Cd(II)-MOFs, [Cd 2 (L1)-(BDC) 2 •1.5i-PrOH] n (1) and [Cd(L2) 0.5 (BDC)(H 2 O)] n (2), with distinct sensing performances are successfully synthesized by pyridyl/pyrimidyl-containing functional ligands 9,10-bis(di-(pyridine-4-yl)methylene)-9,10-dihydroanthracene (L1) and 9,10bis(di(pyrimidin-5-yl)methylene)-9,10-dihydroanthracene (L2). 1 exhibits a 3D (4,6,10)-connected multicylindrical framework with compartments, constructed by 4-connected L1 and BDC 2− in modes A and B, 6-connected Cd1, and 10-connected [Cd 2 (COO) 2 ] 2+ . 2 is fabricated by 4-connected BDC 2− , 7connected Cd, and L2 bridges to generate a 3D (4,7)-connected pillar-layered framework with uncoordinated pyrimidyl N active sites. More importantly, their topologies have not been reported thus far. 1 and 2 have excellent water, pH, and thermal stabilities. 1 can efficiently sense TNP and MDZ in H 2 O, but its Al 3+ sensing ability is relatively average. In sharp contrast, 2 has ultrahigh Al 3+ sensitivity. Its limit of detection (LOD) toward Al 3+ (2.93 × 10 −7 M) is nearly 2 orders of magnitude and 25 times lower than that of 1 (1.18 × 10 −5 M) and the WHO's maximum Al 3+ limit (7.41 × 10 −6 M) in drinking water, respectively. Their sensing mechanisms and different sensing performances are explored in depth.

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Pyridyl/Pyrimidyl-Containing Ligands Modulating Two Cd(II)-MOFs with Distinct Architectures and Al³⁺ Sensing Abilities

Zhang,

Yue,

Lin

et al. 2024

Inorg. Chem.

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Co(II)-Based 2D Coordination Polymer Featuring Energy Storage and Detection of Aqueous Inorganic Anions

Basree,

Ali,

Nayak

et al. 2024

ACS Omega

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A photochromic metal–organic framework with a rare 3D self-interpenetrated architecture and an ultrahigh MnO₄⁻ sensing ability

Abstract: Photochromic materials have shown a wide range of applications.

Cited by 2 publications

References 56 publications

Pyridyl/Pyrimidyl-Containing Ligands Modulating Two Cd(II)-MOFs with Distinct Architectures and Al³⁺ Sensing Abilities

Pyridyl/Pyrimidyl-Containing Ligands Modulating Two Cd(II)-MOFs with Distinct Architectures and Al³⁺ Sensing Abilities

Co(II)-Based 2D Coordination Polymer Featuring Energy Storage and Detection of Aqueous Inorganic Anions

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A photochromic metal–organic framework with a rare 3D self-interpenetrated architecture and an ultrahigh MnO4− sensing ability

Abstract: Photochromic materials have shown a wide range of applications.

Cited by 2 publications

References 56 publications

Pyridyl/Pyrimidyl-Containing Ligands Modulating Two Cd(II)-MOFs with Distinct Architectures and Al3+ Sensing Abilities

Pyridyl/Pyrimidyl-Containing Ligands Modulating Two Cd(II)-MOFs with Distinct Architectures and Al3+ Sensing Abilities

Co(II)-Based 2D Coordination Polymer Featuring Energy Storage and Detection of Aqueous Inorganic Anions

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Product

Resources

About

A photochromic metal–organic framework with a rare 3D self-interpenetrated architecture and an ultrahigh MnO₄⁻ sensing ability

Pyridyl/Pyrimidyl-Containing Ligands Modulating Two Cd(II)-MOFs with Distinct Architectures and Al³⁺ Sensing Abilities

Pyridyl/Pyrimidyl-Containing Ligands Modulating Two Cd(II)-MOFs with Distinct Architectures and Al³⁺ Sensing Abilities