Abstract. The relative contribution of variations in
meteorological and aerosol initial and boundary conditions to the variability
in modelled cloud properties is investigated with a high-resolution ensemble
(30 members). In the investigated case, moderately deep convection develops
along sea-breeze convergence zones over the southwestern peninsula of the UK.
A detailed analysis of the mechanism of aerosol–cloud interactions in this
case has been presented in the first part of this study
(Miltenberger et al., 2018). The meteorological ensemble (10 members) varies by about a factor of 2 in
boundary-layer moisture convergence, surface precipitation, and cloud
fraction, while aerosol number concentrations are varied by a factor of
100 between the three considered aerosol scenarios. If ensemble members
are paired according to the meteorological initial and boundary conditions,
aerosol-induced changes are consistent across the ensemble. Aerosol-induced
changes in CDNC (cloud droplet number concentration), cloud fraction, cell number and size, outgoing shortwave
radiation (OSR), instantaneous and mean precipitation rates, and precipitation
efficiency (PE) are statistically significant at the 5 % level, but
changes in cloud top height or condensate gain are not. In contrast, if
ensemble members are not paired according to meteorological conditions,
aerosol-induced changes are statistically significant only for CDNC, cell
number and size, outgoing shortwave radiation, and precipitation efficiency.
The significance of aerosol-induced changes depends on the aerosol scenarios
compared, i.e. an increase or decrease relative to the standard scenario. A simple statistical analysis of
the results suggests that a large number of realisations (typically >100)
of meteorological conditions within the uncertainty of a single day are
required for retrieving robust aerosol signals in most cloud properties. Only
for CDNC and shortwave radiation small samples are sufficient. While the results are strictly only valid for the investigated
case, the presented evidence combined with previous studies highlights the
necessity for careful consideration of intrinsic predictability,
meteorological conditions, and co-variability between aerosol and
meteorological conditions in observational or modelling studies on aerosol
indirect effects.