“…Composite methods, in which nanofillers are added to a polymer matrix, have been carried out to fabricate high ε polymeric materials. These nanofillers may be mainly divided into four categories: (1) high ε ceramic nanofillers (e.g., BaTiO 3 , PbZrTiO 3 ) [11][12][13][14][15]; (2) organic dipoles (e.g., N-allyl-N-methyl-p-nitroaniline) [16][17][18][19][20]; (3) high ε organic semiconductor (e.g., CuPc) [21][22][23]; and (4) conductive M A N U S C R I P T A C C E P T E D ACCEPTED MANUSCRIPT 3 nano-carbon fillers (e.g., CNT, GRN) [24][25][26][27]. Approach (1) usually requires high loading fractions (>50%) to effectively improve ε, and thus produces the large increase in elastic modulus.…”