A role of a picosecond strain in an ultrafast optically-driven phase transition in VO₂ nanostructures

Abstract

We report on experimental picosecond acoustic studies of an ultrafast photoinduced insulator-to-metal and structural transition in VO2 nanostructures epitaxially grown on Al2O3 substrates with different orientations. Applying a pump-probe technique with combined excitation of a sample with picosecond strain and femtosecond laser pulses we demonstrate that dynamical strain of moderate amplitude of 0.1% has a pronounced impact on ultrafast photoinduced phase transition in VO2 nanohillocks. This enables novel path for controlling such transitions at picosecond and nanometer scales. Our experiments also allowed characterizing elastic and photo-elastic properties of the photo-induced metallic phase in VO2 and to relate them to the properties of the equilibrium phase. Furthermore, we demonstrate the generation of picosecond strain pulses upon laser-induced excitation of thin epitaxial VO2.