Whereas 3D optical motion capture (OMC) systems are considered the gold standard for kinematic assessment in sport science, they present some drawbacks that limit its use in the field. Inertial measurement units (IMUs) incorporating gyroscopes have been considered as a more practical alternative. Thus, the aim of the study was to evaluate the level of agreement for angular velocity between IMU gyroscopes and an OMC system for varying tennis strokes and intensities. In total, 240 signals of angular velocity from different body segments and types of strokes (forehand, backhand and service) were recorded from four players (two competition players and two beginners). The angular velocity of the IMU gyroscopes was compared to the angular velocity from the OMC system. Level of agreement was evaluated by correlation coefficients, magnitudes of errors in absolute and relative values and Bland-Altman plots. Differences between both systems were highly consistent within players’ skill (i.e. along the broad range of velocities) and axes ( x, y, z). Correlations ranged from 0.951 to 0.993, indicating a very strong relationship and concordance. The magnitude of the differences ranged from 4.4 to 35.4 deg·s−1. The difference relative to the maximum angular velocity achieved was less than 5.0%. The study concluded that IMUs and OMC systems showed comparable values. Thus, IMUs seem to be a valid alternative to detect meaningful differences in angular velocity during tennis groundstrokes in field-based experimentation.