2023
DOI: 10.1002/ange.202308780
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A Single‐Crystal Monomer to Single‐Crystal Polymer Reaction Activated by a Triplet Excimer in a Zipper Mechanism

Abstract: A combined experimental and theoretical study focused on the elucidation of the polymerization mechanism of crystal monomer to crystal polymer reaction of a bisindacene compound in the solid state has been carried out. The experimental description and characterization of the polymer product have been reported elsewhere and, in this article, we address the first detailed description of the polymerization process. This reaction pathway consists in the initial formation of a triplet excimer state that relaxes to … Show more

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