Abstract. In the past decade, ozone (O3) pollution has become a severe
environmental problem in China's major cities. Here, based on available
observational records, we investigated the long-term trend of O3
pollution in China during 2014–2020. The O3 concentrations were slightly
higher in urban areas than in non-urban areas. During these 7 years, the
highest O3 concentrations primarily occurred during summer in northern China,
and during autumn or spring in southern China. Although O3 precursors,
including nitrogen oxides (NOx) and carbon monoxide (CO), continuously
decreased, O3 concentrations generally increased throughout the 7
years with a slower increasing rate after 2017. The long-term trend of O3
concentrations differed across seasons, especially from 2019 to 2020, when
O3 concentrations decreased in summer and increased in winter. To analyse
the causes of this observed trend, a photochemical box model was used to
investigate the change in the O3 sensitivity regime in two representative
cities – Beijing and Shanghai. Our model simulations suggest that the
summertime O3 sensitivity regime in urban areas of China has changed from
a VOC-limited regime to a transition regime during 2014–2020. By 2020, the
urban photochemistry was in a transition regime in summer but in a
VOC-limited regime in winter. This study helps to understand the distinct
trends of O3 in China and provides insights into efficient future O3
control strategies in different regions and seasons.