This study proposed a novel continuous roll-forming process of elastomer molds, which can control the deformation of the mold using the rolling belt stack combination method. This study analyzed various rolling belt combinations, assembled the system based on simulation and experimental data according to the deformation requirement design, and obtained a controllable microstructure mold rolling belt with tensile deformation. Mold thickness and microstructure size are key microstructure mold deformation parameters. This study designed and assembled a controllable microstructure mold rolling belt-type imprint molding system and conducted a series of experiments. The impact and application of different experimental system operation procedures and fabrication methods of the auxetic structure rolling belt on replication molding were analyzed. The innovative controllable microstructure mold rolling belt-type imprint replication molding technique proposed in this study had a stable and controllable mold deformation mechanism. It can control and replicate molding.