In this study, nanofluids were synthesized using nanoparticles to improve the efficiency of CO 2 geological storage, and visual observation, dynamic light scattering (DLS), fluid miscibility test (FMT), and transmission electron microscopy (TEM) were performed. Visual observation confirmed that the surface-modified SiO 2 was not precipitated at 1 wt% or more and maintained a stable state. DLS and TEM measurements demonstrated that the average particle size at room temperature (25°C) and high temperature (100°C) was 100 nm or less, which is the definition of nanoparticles. After the FMT, the average particle size was 42.5 nm. The synthesized nanofluid was considered to have acquired dispersion stability under high-temperature and high-salinity reservoir conditions.