Let p ∈ [1, ∞], q ∈ (1, ∞), s ∈ Z + := N ∪ {0}, and α ∈ R. In this article, the authors introduce a reasonable version T of the Calderón-Zygmund operator T on J N con ( p,q,s) α (R n ), the special John-Nirenberg-Campanato space via congruent cubes, which when p = ∞ coincides with the Campanato space C α,q,s (R n ). Then the authors prove that T is bounded on, which is a well-known assumption. To this end, the authors find an equivalent version of this assumption. Moreover, the authors show that T can be extended to a unique continuous linear operator on the Hardy-kind space H K con ( p,q,s) α (R n ), the predual space of J N con ( p ,q ,s) α (R n ) with 1 p + 1 p = 1 = 1 q + 1 q , if and only if, for any γ ∈ Z n + with |γ | ≤ s, T * (x γ ) = 0. The main interesting integrands in the latter boundedness are that, to overcome the difficulty caused by that • H K con ( p,q,s)α (R n ) is no longer concave, the authors first find an equivalent