2022
DOI: 10.1002/chem.202104332
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Abnormal Association between Metal−Organic Cages and Counterions Regulated by the Hydration Shells

Abstract: A unique trend in the binding affinity between cationic metal−organic cages (MOCs) and external counteranions in aqueous media was observed. Similar to many macroions, two MOCs, sharing similar structures but carrying different number of charges, self‐assembled into hollow spherical single‐layered blackberry‐type structures through counterion‐mediated attraction. Dynamic and static light scattering and isothermal titration calorimetry measurements confirm the stronger interactions among less charged MOCs and c… Show more

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